Projects funded by the NCN

Information on the principal investigator and host institution

Information of the project and the call

Keywords

Equipment

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Tracking chemical reaction dynamics with ultrafast X-ray spectroscopies: applications to photooxidation and photocatalysis processes

2016/22/E/ST4/00543

Keywords:

photocatalysis photosensitisation X-ray absorption and emission spectroscopies synchrotron radiation XFEL pump-probe techniques ultrashort laser pulses

Descriptors:

  • ST4_7: Electrochemistry, microfluidics in chemistry, sensors
  • ST4_17: Chemical reactions: mechanisms, thermodynamics, kinetics
  • ST4_3: Molecular architecture and structure

Panel:

ST4 - Chemistry: physical chemistry/chemical physics, theoretical chemistry, analytical chemistry, inorganic chemistry, organic chemistry, method development

Host institution :

Uniwersytet im. Adama Mickiewicza w Poznaniu, Wydział Fizyki

woj. wielkopolskie

Other projects carried out by the institution 

Principal investigator (from the host institution):

dr Wojciech Gawełda 

Number of co-investigators in the project: 6

Call: SONATA BIS 6 - announced on 2016-06-15

Amount awarded: 1 737 784 PLN

Project start date (Y-m-d): 2017-05-15

Project end date (Y-m-d): 2023-05-14

Project duration:: 72 months (the same as in the proposal)

Project status: Project settled

Project description

Download the project description in a pdf file

Note - project descriptions were prepared by the authors of the applications themselves and placed in the system in an unchanged form.

Equipment purchased [PL]

  1. Komórka przepływowa.
  2. Pompka perystaltyczna.
  3. Suszarka laboratoryjna.
  4. Cylindryczne krysztaly dyfrakcyjne do rentgenowskiego spektrometru emisyjnego (wykonane z Si lub Ge) (3 szt.) (108 000 PLN)
  5. Dygestorium.
  6. Sprzęt komputerowy-monitory.
  7. Sprzęt komputerowy-notebooki.
  8. Pompka zębata.
  9. Dewar-pojemnik na ciekły azot.

Information in the final report

  • Publication in academic press/journals (19)
  1. Atomic-scale observation of solvent reorganization influencing photoinduced structural dynamics in a copper complex photosensitizer
    Authors:
    Tetsuo Katayama, Tae-Kyu Choi, Dmitry Khakhulin, Asmus O. Dohn, Christopher J. Milne, Gyorgy Vanko, Zoltan Nemeth, Frederico A. Lima, Jakub Szlachetko, Tokushi Sato, Shunsuke Nozawa, Shin-ichi Adachi, Makina Yabashi, Thomas J. Penfold, Wojciech Gawelda, Gianluca Levi
    Academic press:
    Chemical Science (rok: 2023, tom: 14, strony: 2572-2584), Wydawca: Royal Society of Chemistry
    Status:
    Published
    DOI:
    10.1039/d2sc06600a - link to the publication
  2. Direct observation of nuclear reorganization driven by ultrafast spin transitions
    Authors:
    Yifeng Jiang, Lai Chung Liu, Antoine Sarracini, Kamil M. Krawczyk, Jordan S. Wentzell, Cheng Lu, Ryan L. Field, Samir F. Matar, Wojciech Gawelda, Henrike M. Müller-Werkmeister, R.J.Dwayne Miller
    Academic press:
    Nature Communications (rok: 2020, tom: 11, strony: 1530), Wydawca: Nature Publishing Group
    Status:
    Published
    DOI:
    10.1038/s41467-020-15187-y - link to the publication
  3. Revealing Hot and Long-Lived Metastable Spin States in the Photoinduced Switching of Solvated Metallogrid Complexes with Femtosecond Optical and X‑ray Spectroscopies
    Authors:
    Maria A. Naumova, Aleksandr Kalinko, Joanne W. L. Wong, Mohamed Abdellah, Huifang Geng, Edoardo Domenichini, Jie Meng, Sol Alvarez Gutierrez, Pierre-Adrien Mante, Weihua Lin, Peter Zalden, Andreas Galler, Frederico Lima, Katharina Kubicek, Mykola Biednov, Alexander Britz, Stefano Checchia, Victoria Kabanova, Michael Wulff, Jennifer Zimara, Dirk Schwarzer, Serhiy Demeshko, Vadim Murzin, David Gosztola, Martin Jarenmark, Jianxin Zhang, Matthias Bauer, Max Latevi Lawson Daku, Wojciech Gawelda, Dmitry Khakhulin, Christian Bressler, Franc Meyer, Kaibo Zheng, Sophie E. Canton
    Academic press:
    Journal of Physical Chemistry Letters (rok: 2020, tom: 11, strony: 2133-2141), Wydawca: American Chemical Society
    Status:
    Published
    DOI:
    10.1021/acs.jpclett.9b03883 - link to the publication
  4. Ultrafast Energy Transfer from Photoexcited Tryptophan to the Haem in Cytochrome c
    Authors:
    Camila Bacellar, Jérémy R. Rouxel, Rebecca A. Ingle, Giulia F. Mancini, Dominik Kinschel, Oliviero Cannelli, Yang Zhao, Claudio Cirelli, Gregor Knopp, Jakub Szlachetko, Frederico A. Lima, Samuel Menzi, Dmitry Ozerov, Georgios Pamfilidis, Katharina Kubicek, Dmitry Khakhulin, Wojciech Gawelda, Angel Rodriguez-Fernandez, Mykola Biednov, Christian Bressler, Christopher A. Arrell, Philip J. M. Johnson, Christopher J. Milne, Majed Chergui
    Academic press:
    The Journal of Physical Chemistry Letters (rok: 2023, tom: 14, strony: 2425−2432), Wydawca: American Chemical Society
    Status:
    Published
    DOI:
    10.1021/acs.jpclett.3c00218 - link to the publication
  5. Ultrafast Jahn-Teller Photoswitching in Cobalt Single-Ion Magnets
    Authors:
    Sophie E. Canton, Mykola Biednov, Mátyás Pápai, Frederico A. Lima, Tae-Kyu Choi, Florian Otte, Yifeng Jiang, Paul Frankenberger, Martin Knoll, Peter Zalden, Wojciech Gawelda, Ahibur Rahaman, Klaus B. Møller, Christopher Milne, David J. Gosztola, Kaibo Zheng, Marius Retegan, Dmitry Khakhulin
    Academic press:
    Advanced Science (rok: 2023, tom: 2206880, strony: 2206880), Wydawca: Wiley-VCH Gmbh
    Status:
    Published
    DOI:
    10.1002/advs.202206880 - link to the publication
  6. Elucidation of the photoaquation reaction mechanism in ferrous hexacyanide using synchrotron x-rays with sub-pulse-duration sensitivity
    Authors:
    Anne Marie March , Gilles Doumy, Amity Andersen, Andre Al Haddad, Yoshiaki Kumagai , MingFeng Tu, Joohee Bang, Christoph Bostedt, Jens Uhlig , Daniel R. Nascimento, Tadesse A. Assefa Zoltán Németh , György Vankó , Wojciech Gawelda , Niranjan Govind , Linda Young
    Academic press:
    Journal of Chemical Physics (rok: 2019, tom: 151, strony: 144306), Wydawca: AIP Publishing
    Status:
    Published
    DOI:
    10.1063/1.5117318 - link to the publication
  7. Revealing hole trapping in zinc oxide nanoparticles by time-resolved X-ray spectroscopy
    Authors:
    Thomas J. Penfold, Jakub Szlachetko, Fabio G. Santomauro, Alexander Britz, Wojciech Gawelda, Gilles Doumy, Anne Marie March, Stephen H. Southworth, Jochen Rittmann, Rafael Abela, Majed Chergui, Christopher J. Milne
    Academic press:
    Nature Communications (rok: 2018, tom: 9, strony: 478), Wydawca: Nature Publishing Group
    Status:
    Published
    DOI:
    10.1038/s41467-018-02870-4 - link to the publication
  8. Ultrafast two-colour X-ray emission spectroscopy reveals excited state landscape in a base metal dyad
    Authors:
    M. Nowakowski, M. Huber-Gedert, H. Elgabarty, J. Kubicki, A. Kertem, N. Lindner, D. Khakhulin, F. Lima, T.-K. Choi, M. Biednov, N. Piergies, P. Zalden, K. Kubicek, A. Rodriguez-Fernandez, M. Alaraby Salem, T. Kühne, W. Gawelda, M. Bauer
    Academic press:
    Nature Communications (rok: 2023, ), Wydawca: Nature Publishing Group
    Status:
    Submitted
    DOI:
    10.48550/arXiv.2301.04425 - link to the publication
  9. A sensitive high repetition rate arrival time monitor for X-ray Free Electron Lasers
    Authors:
    Michael Diez, Henning Kirchberg, Andreas Galler, Sebastian Schulz, Mykola Biednov, Christina Boemer, Tae-Kyu Choi, Angel Rodriguez-Fernandez, Wojciech Gawelda, Dmitry Khakhulin, Katharina Kubicek, Frederico Lima, Florian Otte, Peter Zalden, Ryan Coffee, Michael Thorwart, Christian Bressler
    Academic press:
    Nature Communications (rok: 2023, tom: 14, strony: 2495), Wydawca: Nature Publishing Group
    Status:
    Published
    DOI:
    10.1038/s41467-023-38143-y - link to the publication
  10. Site-Selective Real-Time Observation of Bimolecular Electron Transfer in a Photocatalytic System Using L-Edge X-Ray Absorption Spectroscopy
    Authors:
    Alexander Britz, Sergey I Bokarev, Tadesse A Assefa, Èva G Bajnóczi, Zoltán Németh, György Vankó, Nils Rockstroh, Henrik Junge, Matthias Beller, Gilles Doumy, Anne Marie March, Stephen H Southworth, Stefan Lochbrunner, Oliver Kühn, Christian Bressler, Wojciech Gawełda
    Academic press:
    ChemPhysChem (rok: 2021, tom: 22, strony: 693-700), Wydawca: Wiley-VCH GmbH, Weinheim
    Status:
    Published
    DOI:
    10.1002/cphc.202000845 - link to the publication
  11. Unveiling the origin of photo-induced enhancement of oxidation catalysis at Mo(VI) centres of Ru(II)–Mo(VI) dyads
    Authors:
    Maryam Nazari Haghighi Pashaki, Tae-Kyu Choi, Egmont J. Rohwer, Thomas Feurer, Anne-Kathrin Duhme-Klair, Wojciech Gawełda, Andrea Cannizzo
    Academic press:
    Chemical Communications (rok: 2021, tom: 57, strony: 4142-4145), Wydawca: The Royal Society of Chemistry
    Status:
    Published
    DOI:
    10.1039/D1CC00750E - link to the publication
  12. Combining X-ray Kb1,3, valence-to-core, and X-ray Raman spectroscopy for studying Earth materials at high pressure and temperature: the case of siderite
    Authors:
    Christopher Weis, Georg Spiekermann, Christian Sternemann, Manuel Harder, Gyorgy Vanko, Valerio Cerantola, Christoph J. Sahle, Yury Forov, Robin Sakrowski, Ilya Kupenko, Sylvain Petitgirard, Hasan Yavas, Christian Bressler, Wojciech Gawelda, Metin Tolan, Max Wilke
    Academic press:
    Journal of Analytical Atomic Spectrometry (rok: 2019, tom: 34, strony: 384), Wydawca: Royal Society of Chemistry
    Status:
    Published
    DOI:
    10.1039/c8ja00247a - link to the publication
  13. Exploring the light-induced dynamics in solvated metallogrid complexes with femtosecond pulses across the electromagnetic spectrum
    Authors:
    Maria Naumova, Aleksandr Kalinko, Joanne Wong, Sol Laura Gutierrez Alvarez, Jie Meng, Mingli Liang, Mohamed Abdellah, Huifang Geng, Weihua Lin, Katharina Kubicek, Mykola Biednov, Frederico Lima, Andreas Galler, Peter Zalden, Stefano Checchia, Pierre-Adrien Mante, Jennifer Zimara, Dirk Schwarzer, Serhiy Demeshko, Vadim Murzin, David Gosztola, Martin Jarenmark, Jianxin Zhang, Matthias Bauer, Latevi Max Lawson Daku, Dmitry Khakhulin, Wojciech Gawelda, Christian Bressler, Franc Meyer, Kaibo Zheng, Sophie Canton
    Academic press:
    Journal of Chemical Physics (rok: 2020, tom: 152, strony: 214301), Wydawca: AIP Publishing
    Status:
    Published
    DOI:
    10.1063/1.5138641 - link to the publication
  14. Femtosecond X-ray emission study of the spin cross-over dynamics in heme proteins"
    Authors:
    D. Kinschel, C. Bacellar, O. Cannelli, B. Sorokin , T. Katayama, G. F. Mancini, J. R. Rouxel, Y. Obara, J. Nishitani, H. Ito, T. Ito, N. Kurahashi, C. Higashimura, S. Kudo, T. Keane, F. A. Lima, W. Gawelda, P. Zalden, S. Schulz, J. Budarz, D. Khakhulin, A. Galler, C. Bressler, C. J. Milne, T. Penfold, M. Yabashi, T. Suzuki, K. Misawa, M. Chergui
    Academic press:
    Nature Communications (rok: 2020, tom: 11, strony: 4145), Wydawca: Nature Publishing Group
    Status:
    Published
    DOI:
    10.1038/s41467-020-17923-w - link to the publication
  15. Fundamental Characterization, Photophysics and Photocatalysis of a Base Metal Iron(II)-Cobalt(III) Dyad
    Authors:
    Marina Huber-Gedert, Michał Nowakowski, Ahmet Kertmen, Lukas Burkhardt, Natalia Lindner, Roland Schoch, Regine Herbst-Irmer, Adam Neuba, Lennart Schmitz, Tae-Kyu Choi, Jacek Kubicki, Wojciech Gawełda, Matthias Bauer
    Academic press:
    Chemistry-A European Journal (rok: 2021, tom: 27, strony: 9905-9918), Wydawca: Wiley-VCH GmbH, Weinheim
    Status:
    Published
    DOI:
    10.1002/chem.202100766 - link to the publication
  16. Spin cascade and doming in ferric hemes: Femtosecond X-ray absorption and X-ray emission studies
    Authors:
    C. Bacellar, D. Kinschel, G. Mancini, R. Ingle, J. Rouxel, O. Cannelli, C. Cirelli, G. Knopp, J. Szlachetko, F. Lima, S. Menzi, G. Pamfilidis, K. Kubicek, D. Khakhulin, W. Gawelda, A. Rodriguez-Fernandez, M. Biednov, C. Bressler, C. Arrell, P. Johnson, C. Milne, M. Chergui
    Academic press:
    Proceedings of the National Academy of Sciences USA (rok: 2020, tom: 117, strony: 21914-21920), Wydawca: National Academy of Sciences of the United States of America
    Status:
    Published
    DOI:
    10.1073/pnas.2009490117 - link to the publication
  17. Towards Noble-Metal-Free Dyads: Ground and Excited State Tuning by a Cobalt Dimethylglyoxime Motif Connected to an Iron N-Heterocyclic Carbene Photosensitizer
    Authors:
    Peter Zimmer, Lukas Burkhardt, Rahel Schepper, Kaibo Zheng, David Gosztola, Adam Neuba, Ulrich Flörke, Christoph Wölper, Roland Schoch, Wojciech Gawelda, Sophie E. Canton, Matthias Bauer
    Academic press:
    European Journal of Inorganic Chemistry (rok: 2018, tom: 2018, strony: 5203–5214), Wydawca: Wiley-VCH Verlag GmbH
    Status:
    Published
    DOI:
    10.1002/ejic.201800946 - link to the publication
  18. Tracking multiple components of a nuclear wavepacket in photoexcited Cu(I)-phenanthroline complex using ultrafast X-ray spectroscopy
    Authors:
    Tetsuo Katayama, Thomas Northey, Wojciech Gawelda, Christopher J. Milne, György Vankó, Frederico A. Lima, Rok Bohinc, Zoltán Németh, Shunsuke Nozawa, Tokushi Sato, Dmitry Khakhulin, Jakub Szlachetko, Tadashi Togashi, Shigeki Owada, Shin-ichi Adachi, Christian Bressler, Makina Yabashi, Thomas J. Penfold
    Academic press:
    Nature Communications (rok: 2019, tom: 10, strony: 3606), Wydawca: Nature Publishing Group
    Status:
    Published
    DOI:
    10.1038/s41467-019-11499-w - link to the publication
  19. Using Ultrafast X‑ray Spectroscopy To Address Questions in LigandField Theory: The Excited State Spin and Structure of [Fe(dcpp)2]2+
    Authors:
    Alexander Britz, Wojciech Gawelda, Tadesse A. Assefa, Lindsey L. Jamula, Jonathan T. Yarranton, Andreas Galler, Dmitry Khakhulin, Michael Diez, Manuel Harder, Gilles Doumy, Anne Marie March, Eva Bajnoczi, Zoltan Nemeth, Matyas Papai, Emese Rozsalyi, Dorottya Szemes, Hana Cho, Sriparna Mukherjee, Chang Liu, Tae Kyu Kim, Robert W. Schoenlein, Stephen H. Southworth, Linda Young, Elena Jakubikova, Nils Huse, György Vankó, Christian Bressler, James K. McCusker
    Academic press:
    Inorganic Chemistry (rok: 2019, tom: 58, strony: 9341-9350), Wydawca: American Chemical Society
    Status:
    Published
    DOI:
    10.1021/acs.inorgchem.9b01063 - link to the publication

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