Tracking chemical reaction dynamics with ultrafast X-ray spectroscopies: applications to photooxidation and photocatalysis processes
2016/22/E/ST4/00543
Keywords
Descriptors
- ST4_7: Fizyka chemiczna
- ST4_17: Fotochemia
- ST4_3: Metody spektroskopowe i spektrometryczne
Panel
ST4 – Chemistry: physical chemistry/chemical physics, theoretical chemistry, analytical chemistry, inorganic chemistry, organic chemistry, method development
Host institution
Uniwersytet im. Adama Mickiewicza w Poznaniu, Wydział Fizyki
Voivodeship: wielkopolskie
Principal investigator (from the host institution)
Number of co-investigators in the project: 6
Call
SONATA BIS 6 – announced on 2016-06-15
- Amount awarded
- 1 737 784 PLN
- Project start date
- 2017-05-15
- Project end date
- 2023-05-14
- Project duration
- 72 months (the same as in the proposal)
- Project status
- Project settled
Project description
Download the project description in a pdf file
Note — project descriptions were prepared by the authors of the applications themselves and placed in the system in an unchanged form.
Equipment purchased [PL]
- Cylindryczne krysztaly dyfrakcyjne do rentgenowskiego spektrometru emisyjnego (wykonane z Si lub Ge) (3 pcs). Cost: 108 000 PLN
- Dewar-pojemnik na ciekły azot.
- Dygestorium.
- Komórka przepływowa.
- Pompka perystaltyczna.
- Pompka zębata.
- Sprzęt komputerowy-monitory.
- Sprzęt komputerowy-notebooki.
- Suszarka laboratoryjna.
Information in the final report
Publication in academic press/journals (18)
-
Fundamental Characterization, Photophysics and Photocatalysis of a Base Metal Iron(II)-Cobalt(III) Dyad
- Authors:
- Marina Huber-Gedert, Michał Nowakowski, Ahmet Kertmen, Lukas Burkhardt, Natalia Lindner, Roland Schoch, Regine Herbst-Irmer, Adam Neuba, Lennart Schmitz, Tae-Kyu Choi, Jacek Kubicki, Wojciech Gawełda, Matthias Bauer
- Academic press:
- Chemistry-A European Journal (year: 2021, volume: 27, pages: 9905-9918), Publisher: Wiley-VCH GmbH, Weinheim
- Status:
- Published
- DOI:
- 10.1002/chem.202100766 – link to the publication
-
Unveiling the origin of photo-induced enhancement of oxidation catalysis at Mo(VI) centres of Ru(II)–Mo(VI) dyads
- Authors:
- Maryam Nazari Haghighi Pashaki, Tae-Kyu Choi, Egmont J. Rohwer, Thomas Feurer, Anne-Kathrin Duhme-Klair, Wojciech Gawełda, Andrea Cannizzo
- Academic press:
- Chemical Communications (year: 2021, volume: 57, pages: 4142-4145), Publisher: The Royal Society of Chemistry
- Status:
- Published
- DOI:
- 10.1039/D1CC00750E – link to the publication
-
Spin cascade and doming in ferric hemes: Femtosecond X-ray absorption and X-ray emission studies
- Authors:
- C. Bacellar, D. Kinschel, G. Mancini, R. Ingle, J. Rouxel, O. Cannelli, C. Cirelli, G. Knopp, J. Szlachetko, F. Lima, S. Menzi, G. Pamfilidis, K. Kubicek, D. Khakhulin, W. Gawelda, A. Rodriguez-Fernandez, M. Biednov, C. Bressler, C. Arrell, P. Johnson, C. Milne, M. Chergui
- Academic press:
- Proceedings of the National Academy of Sciences USA (year: 2020, volume: 117, pages: 21914-21920), Publisher: National Academy of Sciences of the United States of America
- Status:
- Published
- DOI:
- 10.1073/pnas.2009490117 – link to the publication
-
Femtosecond X-ray emission study of the spin cross-over dynamics in heme proteins
- Authors:
- D. Kinschel, C. Bacellar, O. Cannelli, B. Sorokin , T. Katayama, G. F. Mancini, J. R. Rouxel, Y. Obara, J. Nishitani, H. Ito, T. Ito, N. Kurahashi, C. Higashimura, S. Kudo, T. Keane, F. A. Lima, W. Gawelda, P. Zalden, S. Schulz, J. Budarz, D. Khakhulin, A. Galler, C. Bressler, C. J. Milne, T. Penfold, M. Yabashi, T. Suzuki, K. Misawa, M. Chergui
- Academic press:
- Nature Communications (year: 2020, volume: 11, pages: 4145), Publisher: Nature Publishing Group
- Status:
- Published
- DOI:
- 10.1038/s41467-020-17923-w – link to the publication
-
Ultrafast Energy Transfer from Photoexcited Tryptophan to the Haem in Cytochrome c
- Authors:
- Camila Bacellar, Jérémy R. Rouxel, Rebecca A. Ingle, Giulia F. Mancini, Dominik Kinschel, Oliviero Cannelli, Yang Zhao, Claudio Cirelli, Gregor Knopp, Jakub Szlachetko, Frederico A. Lima, Samuel Menzi, Dmitry Ozerov, Georgios Pamfilidis, Katharina Kubicek, Dmitry Khakhulin, Wojciech Gawelda, Angel Rodriguez-Fernandez, Mykola Biednov, Christian Bressler, Christopher A. Arrell, Philip J. M. Johnson, Christopher J. Milne, Majed Chergui
- Academic press:
- The Journal of Physical Chemistry Letters (year: 2023, volume: 14, pages: 2425−2432), Publisher: American Chemical Society
- Status:
- Published
- DOI:
- 10.1021/acs.jpclett.3c00218 – link to the publication
-
A sensitive high repetition rate arrival time monitor for X-ray Free Electron Lasers
- Authors:
- Michael Diez, Henning Kirchberg, Andreas Galler, Sebastian Schulz, Mykola Biednov, Christina Boemer, Tae-Kyu Choi, Angel Rodriguez-Fernandez, Wojciech Gawelda, Dmitry Khakhulin, Katharina Kubicek, Frederico Lima, Florian Otte, Peter Zalden, Ryan Coffee, Michael Thorwart, Christian Bressler
- Academic press:
- Nature Communications (year: 2023, volume: 14, pages: 2495), Publisher: Nature Publishing Group
- Status:
- Published
- DOI:
- 10.1038/s41467-023-38143-y – link to the publication
-
Site-Selective Real-Time Observation of Bimolecular Electron Transfer in a Photocatalytic System Using L-Edge X-Ray Absorption Spectroscopy
- Authors:
- Alexander Britz, Sergey I Bokarev, Tadesse A Assefa, Èva G Bajnóczi, Zoltán Németh, György Vankó, Nils Rockstroh, Henrik Junge, Matthias Beller, Gilles Doumy, Anne Marie March, Stephen H Southworth, Stefan Lochbrunner, Oliver Kühn, Christian Bressler, Wojciech Gawełda
- Academic press:
- ChemPhysChem (year: 2021, volume: 22, pages: 693-700), Publisher: Wiley-VCH GmbH, Weinheim
- Status:
- Published
- DOI:
- 10.1002/cphc.202000845 – link to the publication
-
Atomic-scale observation of solvent reorganization influencing photoinduced structural dynamics in a copper complex photosensitizer
- Authors:
- Tetsuo Katayama, Tae-Kyu Choi, Dmitry Khakhulin, Asmus O. Dohn, Christopher J. Milne, Gyorgy Vanko, Zoltan Nemeth, Frederico A. Lima, Jakub Szlachetko, Tokushi Sato, Shunsuke Nozawa, Shin-ichi Adachi, Makina Yabashi, Thomas J. Penfold, Wojciech Gawelda, Gianluca Levi
- Academic press:
- Chemical Science (year: 2023, volume: 14, pages: 2572-2584), Publisher: Royal Society of Chemistry
- Status:
- Published
- DOI:
- 10.1039/d2sc06600a – link to the publication
-
Combining X-ray Kb1,3, valence-to-core, and X-ray Raman spectroscopy for studying Earth materials at high pressure and temperature: the case of siderite
- Authors:
- Christopher Weis, Georg Spiekermann, Christian Sternemann, Manuel Harder, Gyorgy Vanko, Valerio Cerantola, Christoph J. Sahle, Yury Forov, Robin Sakrowski, Ilya Kupenko, Sylvain Petitgirard, Hasan Yavas, Christian Bressler, Wojciech Gawelda, Metin Tolan, Max Wilke
- Academic press:
- Journal of Analytical Atomic Spectrometry (year: 2019, volume: 34, pages: 384), Publisher: Royal Society of Chemistry
- Status:
- Published
- DOI:
- 10.1039/c8ja00247a – link to the publication
-
Elucidation of the photoaquation reaction mechanism in ferrous hexacyanide using synchrotron x-rays with sub-pulse-duration sensitivity
- Authors:
- Anne Marie March , Gilles Doumy, Amity Andersen, Andre Al Haddad, Yoshiaki Kumagai , MingFeng Tu, Joohee Bang, Christoph Bostedt, Jens Uhlig , Daniel R. Nascimento, Tadesse A. Assefa Zoltán Németh , György Vankó , Wojciech Gawelda , Niranjan Govind , Linda Young
- Academic press:
- Journal of Chemical Physics (year: 2019, volume: 151, pages: 144306), Publisher: AIP Publishing
- Status:
- Published
- DOI:
- 10.1063/1.5117318 – link to the publication
-
Ultrafast Jahn-Teller Photoswitching in Cobalt Single-Ion Magnets
- Authors:
- Sophie E. Canton, Mykola Biednov, Mátyás Pápai, Frederico A. Lima, Tae-Kyu Choi, Florian Otte, Yifeng Jiang, Paul Frankenberger, Martin Knoll, Peter Zalden, Wojciech Gawelda, Ahibur Rahaman, Klaus B. Møller, Christopher Milne, David J. Gosztola, Kaibo Zheng, Marius Retegan, Dmitry Khakhulin
- Academic press:
- Advanced Science (year: 2023, volume: 2206880, pages: 2206880), Publisher: Wiley-VCH Gmbh
- Status:
- Published
- DOI:
- 10.1002/advs.202206880 – link to the publication
-
Towards Noble-Metal-Free Dyads: Ground and Excited State Tuning by a Cobalt Dimethylglyoxime Motif Connected to an Iron N-Heterocyclic Carbene Photosensitizer
- Authors:
- Peter Zimmer, Lukas Burkhardt, Rahel Schepper, Kaibo Zheng, David Gosztola, Adam Neuba, Ulrich Flörke, Christoph Wölper, Roland Schoch, Wojciech Gawelda, Sophie E. Canton, Matthias Bauer
- Academic press:
- European Journal of Inorganic Chemistry (year: 2018, volume: 2018, pages: 5203–5214), Publisher: Wiley-VCH Verlag GmbH
- Status:
- Published
- DOI:
- 10.1002/ejic.201800946 – link to the publication
-
Tracking multiple components of a nuclear wavepacket in photoexcited Cu(I)-phenanthroline complex using ultrafast X-ray spectroscopy
- Authors:
- Tetsuo Katayama, Thomas Northey, Wojciech Gawelda, Christopher J. Milne, György Vankó, Frederico A. Lima, Rok Bohinc, Zoltán Németh, Shunsuke Nozawa, Tokushi Sato, Dmitry Khakhulin, Jakub Szlachetko, Tadashi Togashi, Shigeki Owada, Shin-ichi Adachi, Christian Bressler, Makina Yabashi, Thomas J. Penfold
- Academic press:
- Nature Communications (year: 2019, volume: 10, pages: 3606), Publisher: Nature Publishing Group
- Status:
- Published
- DOI:
- 10.1038/s41467-019-11499-w – link to the publication
-
Revealing Hot and Long-Lived Metastable Spin States in the Photoinduced Switching of Solvated Metallogrid Complexes with Femtosecond Optical and X‑ray Spectroscopies
- Authors:
- Maria A. Naumova, Aleksandr Kalinko, Joanne W. L. Wong, Mohamed Abdellah, Huifang Geng, Edoardo Domenichini, Jie Meng, Sol Alvarez Gutierrez, Pierre-Adrien Mante, Weihua Lin, Peter Zalden, Andreas Galler, Frederico Lima, Katharina Kubicek, Mykola Biednov, Alexander Britz, Stefano Checchia, Victoria Kabanova, Michael Wulff, Jennifer Zimara, Dirk Schwarzer, Serhiy Demeshko, Vadim Murzin, David Gosztola, Martin Jarenmark, Jianxin Zhang, Matthias Bauer, Max Latevi Lawson Daku, Wojciech Gawelda, Dmitry Khakhulin, Christian Bressler, Franc Meyer, Kaibo Zheng, Sophie E. Canton
- Academic press:
- Journal of Physical Chemistry Letters (year: 2020, volume: 11, pages: 2133-2141), Publisher: American Chemical Society
- Status:
- Published
- DOI:
- 10.1021/acs.jpclett.9b03883 – link to the publication
-
Exploring the light-induced dynamics in solvated metallogrid complexes with femtosecond pulses across the electromagnetic spectrum
- Authors:
- Maria Naumova, Aleksandr Kalinko, Joanne Wong, Sol Laura Gutierrez Alvarez, Jie Meng, Mingli Liang, Mohamed Abdellah, Huifang Geng, Weihua Lin, Katharina Kubicek, Mykola Biednov, Frederico Lima, Andreas Galler, Peter Zalden, Stefano Checchia, Pierre-Adrien Mante, Jennifer Zimara, Dirk Schwarzer, Serhiy Demeshko, Vadim Murzin, David Gosztola, Martin Jarenmark, Jianxin Zhang, Matthias Bauer, Latevi Max Lawson Daku, Dmitry Khakhulin, Wojciech Gawelda, Christian Bressler, Franc Meyer, Kaibo Zheng, Sophie Canton
- Academic press:
- Journal of Chemical Physics (year: 2020, volume: 152, pages: 214301), Publisher: AIP Publishing
- Status:
- Published
- DOI:
- 10.1063/1.5138641 – link to the publication
-
Using Ultrafast X‑ray Spectroscopy To Address Questions in LigandField Theory: The Excited State Spin and Structure of [Fe(dcpp)2]2+
- Authors:
- Alexander Britz, Wojciech Gawelda, Tadesse A. Assefa, Lindsey L. Jamula, Jonathan T. Yarranton, Andreas Galler, Dmitry Khakhulin, Michael Diez, Manuel Harder, Gilles Doumy, Anne Marie March, Eva Bajnoczi, Zoltan Nemeth, Matyas Papai, Emese Rozsalyi, Dorottya Szemes, Hana Cho, Sriparna Mukherjee, Chang Liu, Tae Kyu Kim, Robert W. Schoenlein, Stephen H. Southworth, Linda Young, Elena Jakubikova, Nils Huse, György Vankó, Christian Bressler, James K. McCusker
- Academic press:
- Inorganic Chemistry (year: 2019, volume: 58, pages: 9341-9350), Publisher: American Chemical Society
- Status:
- Published
- DOI:
- 10.1021/acs.inorgchem.9b01063 – link to the publication
-
Direct observation of nuclear reorganization driven by ultrafast spin transitions
- Authors:
- Yifeng Jiang, Lai Chung Liu, Antoine Sarracini, Kamil M. Krawczyk, Jordan S. Wentzell, Cheng Lu, Ryan L. Field, Samir F. Matar, Wojciech Gawelda, Henrike M. Müller-Werkmeister, R.J.Dwayne Miller
- Academic press:
- Nature Communications (year: 2020, volume: 11, pages: 1530), Publisher: Nature Publishing Group
- Status:
- Published
- DOI:
- 10.1038/s41467-020-15187-y – link to the publication
-
Revealing hole trapping in zinc oxide nanoparticles by time-resolved X-ray spectroscopy
- Authors:
- Thomas J. Penfold, Jakub Szlachetko, Fabio G. Santomauro, Alexander Britz, Wojciech Gawelda, Gilles Doumy, Anne Marie March, Stephen H. Southworth, Jochen Rittmann, Rafael Abela, Majed Chergui, Christopher J. Milne
- Academic press:
- Nature Communications (year: 2018, volume: 9, pages: 478), Publisher: Nature Publishing Group
- Status:
- Published
- DOI:
- 10.1038/s41467-018-02870-4 – link to the publication