Projects funded by the NCN


Information on the principal investigator and host institution

Information of the project and the call

Keywords

Equipment

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New base catalysts active in the production of biodiesel and fine-chemicals

2014/15/B/ST5/00167

Keywords:

mesoporous materials generation of basic centres characteristic transesterification of vegetable oils receiving of fine chemicals

Descriptors:

  • ST5_3: Surface modification
  • ST5_18:
  • ST5_6: Porous materials, ceramics, glasses

Panel:

ST5 - Materials: materials synthesis, structure-properties relations, advanced and functional materials with designed properties, (macro)molecular architecture, material engineering

Host institution :

Uniwersytet im. Adama Mickiewicza w Poznaniu, Wydział Chemii

woj. wielkopolskie

Other projects carried out by the institution 

Principal investigator (from the host institution):

prof. Maria Ziółek 

Number of co-investigators in the project: 9

Call: OPUS 8 - announced on 2014-09-15

Amount awarded: 938 100 PLN

Project start date (Y-m-d): 2015-07-20

Project end date (Y-m-d): 2018-07-19

Project duration:: 36 months (the same as in the proposal)

Project status: Project settled

Equipment purchased [PL]

  1. Waga analityczna (27 000 PLN)
  2. Chromatograf gazowy (92 988 PLN)
  3. reaktor do prowadzenia procesów katalitycznych w fazie ciekłej (200 000 PLN)

Information in the final report

  • Publication in academic press/journals (19)
  • Articles in post-conference publications (33)
  • Book publications / chapters in book publications (2)
  1. Formation of Pt–Ag alloy on different silicas – surface properties and catalytic activity in oxidation of methanol
    Authors:
    J. Wisniewska, M. Ziolek
    Academic press:
    RSC Advances (rok: 2017, tom: 7, strony: 9534–9544), Wydawca: Royal Society of Chemistry
    Status:
    Published
    DOI:
    10.1039/c6ra28365a - link to the publication
  2. MWW layered zeolites modified with niobium species - surface and catalytic properties
    Authors:
    Anna Wojtaszek-Gurdak, Martyna Zielinska, Maria Ziolek
    Academic press:
    Catalysis Today (rok: 2019, tom: 325, strony: 89-97), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.cattod.2018.07.044 - link to the publication
  3. Mesoporous niobosilicate NbMCF modified with alkali metals in the synthesis of chromene derivatives
    Authors:
    A. Smuszkiewicz, J. Lopez-Sanz, I. Sobczak, M. Ziolek, R.M. Martin-Aranda, E. Soriano, E. Perez-Mayoral
    Academic press:
    Catalysis Today (rok: 2016, tom: 277, strony: 133-142), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.cattod.2016.02.042 - link to the publication
  4. Mobility of gold, copper and cerium species in Au, Cu/Ce, Zr-oxides and its impact on total oxidation of methanol
    Authors:
    P. Kaminski, M. Ziolek
    Academic press:
    Applied Catalysis B, Environmental (rok: 2016, tom: 187, strony: 328-341), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.apcatb.2016.01.040 - link to the publication
  5. Tantalum vs Niobium MCF nanocatalysts in the green synthesis of chromene derivatives
    Authors:
    Agata Smuszkiewicz, Jesús López-Sanza, Izabela Sobczak, Rosa M. Martín-Aranda, Maria Ziolek, Elena Pérez-Mayoral
    Academic press:
    Catalysis Today (rok: 2019, tom: 325, strony: 47-52), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.cattod.2018.06.038 - link to the publication
  6. Development of basicity in mesoporous silicas and metallosilicates
    Authors:
    D. Kryszak, K. Stawicka, M. Trejda, V. Calvino-Casilda, R. Martin-Aranda, M. Ziolek
    Academic press:
    Catal. Sci. Technol. (rok: 2017, tom: 7, strony: 5236 - 5248), Wydawca: Royal Society of Chemistry
    Status:
    Published
    DOI:
    10.1039/C7CY00927E - link to the publication
  7. Imidazole immobilization in nanopores of silicas and niobiosilicates SBA-15 and MCF—A new concept towards creation of basicity
    Authors:
    D. Kryszak, K. Stawicka, V. Calvino-Casilda, R.M. Martin-Aranda, M. Ziolek
    Academic press:
    Applied Catalysis A General (rok: 2017, tom: 531, strony: 139-150), Wydawca: Elsevier
    Status:
    Published
  8. Insight into the interaction of calcium species with mesoporous silica and niobiosilica
    Authors:
    Maciej Trejda, Dorota Kryszak, Maria Ziolek
    Academic press:
    Materials Research Bulletin (rok: 2018, tom: 97, strony: 530-536), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.materresbull.2017.09.050 - link to the publication
  9. Supported and inserted monomeric niobium oxide species on/in silica: a molecular picture
    Authors:
    D.C. Tranca, A. Wojtaszek-Gurdak, M. Ziolek, F. Tielens
    Academic press:
    Phys. Chem. Chem. Phys. (rok: 2015, tom: 17, strony: 22401-22411), Wydawca: Royal Society of Chemistry
    Status:
    Published
    DOI:
    101039/c55cp03450g - link to the publication
  10. The effect of structure of mesoporous silica and niobiosilicate on incorporation and stability of modifiers introduced by the click reaction catalyzed by different copper salts
    Authors:
    Katarzyna Stawicka, Klaudia Drazkiewicz, Maria Ziolek
    Academic press:
    Microporous & Mesoporous Materials (rok: 2018, tom: 258, strony: 41-54), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.micromeso.2017.09.005 - link to the publication
  11. The role of gold dopant in AP-Nb/MCF and AP-MCF on the Knoevenagel condensation of ethyl cyanoacetate with benzaldehyde and 2,4-dichlorobenzaldehyde
    Authors:
    Izabela Sobczak, Vanesa Calvino-Casilda, Lukasz Wolski, Tomasz Siodla, Rosa Martin-Aranda, Maria Ziolek
    Academic press:
    Catalysis Today (rok: 2019, tom: 325, strony: 81-88), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.cattod.2018.07.035 - link to the publication
  12. The role of metallic modifiers of SBA-15 supports for propyl-amines on activity and selectivity in the Knoevenagel reactions
    Authors:
    V. Calvino-Casilda, M. Olejniczak, R.M. Martin-Aranda, M. Ziolek
    Academic press:
    Microporous Mesoporous Mater. (rok: 2016, tom: 224, strony: 201-207), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.micromeso.2015.11.027 - link to the publication
  13. The role of niobium component in heterogeneous catalysts
    Authors:
    M. Ziolek, I. Sobczak
    Academic press:
    Catalysis Today (rok: 2017, tom: 285, strony: 211-225), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.cattod.2016.12.013 - link to the publication
  14. Ca/MCF catalysts — The impact of niobium and material structure on basicity
    Authors:
    Dorota Kryszak, Maciej Trejda, Natalia Benedyczak, Maria Ziolek
    Academic press:
    Catalysis Today (rok: 2019, tom: 325, strony: 45613), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.cattod.2018.05.054 - link to the publication
  15. Comparative study of acid-basic properties of MCF impregnated with niobium and cerium species
    Authors:
    Katarzyna Stawicka, Piotr Decyk, Anna Wojtaszek-Gurdak, Maria Ziolek
    Academic press:
    Catalysis Today (rok: 2019, tom: 325, strony: 45332), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.cattod.2018.05.025 - link to the publication
  16. Development of multifunctional gold, copper, zinc, niobium containing MCF catalysts - Surface properties and activity in methanol oxidation
    Authors:
    3.L. Wolski, I. Sobczak, M. Ziolek
    Academic press:
    Microporous Mesoporous Materials (rok: 2017, tom: 243, strony: 339-350), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.micromeso.2017.02.038 - link to the publication
  17. Impact of Brønsted acid sites in MWW zeolites modified with cesium and amine species on Knoevenagel condensation
    Authors:
    Anna Wojtaszek-Gurdak, Vanesa Calvino-Casilda, Aneta Grzelak, Rosa Martin-Aranda, Maria Ziolek
    Academic press:
    Microporous and Mesoporous Materials (rok: 2019, tom: 280, strony: 288-296), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.micromeso.2019.02.007 - link to the publication
  18. The effect of niobium and tantalum on physicochemical and catalytic properties of silver and platinum catalysts based on MCF mesoporous cellular foams
    Authors:
    J. Wisniewska, M. Ziolek, N. Artioli, M. Daturi
    Academic press:
    Journal of Catalysis (rok: 2016, tom: 336, strony: 58-75), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.cat.2015.12.018 - link to the publication
  19. UV-Vis spectroscopy combined with azastilbene probe as a tool for testing basicity of mesoporous silica modified with nitrogen compounds
    Authors:
    Katarzyna Stawicka, Dorota Prukała, Tomasz Siodła, Marek Sikorski, Maria Ziolek
    Academic press:
    Applied Catalysis A (rok: 2019, tom: 570, strony: 339-347), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.apcata.2018.12.003 - link to the publication
  1. Comparative study of Basic oxygen form on MCF impregnation with niobium and cerium species – NO as a probe molecule
    Authors:
    K. Stawicka, P. Decyk, A. Wojtaszek-Gurdak, M. Ziolek
    Conference:
    9th International Symposium on Group Five Elements (rok: 2017, ), Wydawca: Indian Institute of Technology, Kanpur
    Data:
    konferencja 22-24.11
    Status:
    Published
  2. Insight into the interaction between calcium species with mesoporous silica and niobiosilica
    Authors:
    D. Kryszak, K. Stawicka, V. Calvino-Casilda, R.M. Martin-Aranda, M. Trejda
    Conference:
    XXI Forum Zeolitowe (rok: 2017, ), Wydawca: ISBN: 678-83-62783-10-6
    Data:
    konferencja 7-11.02
    Status:
    Published
  3. Insight into the interaction of calcium species with mesoporous silica and niobiosilica
    Authors:
    M. Trejda, D. Kryszak, M. Ziolek
    Conference:
    9th International Symposium on Group Five Elements (rok: 2017, ), Wydawca: Indian Institute of Technology, Kanpur
    Data:
    konferencja 22-24.11
    Status:
    Published
  4. Mesoporous molecular sieves of SBA-15 type based on calcium and niobium as basic catalyst
    Authors:
    M. Trejda, D. Kryszak, E. Drgas, A. Zdziabek, M. Ziolek
    Conference:
    18th International Zeolite Conference (rok: 2016, ), Wydawca: Uniwersytet w Rio de Janeiro
    Data:
    konferencja 19 - 24. 06
    Status:
    Published
  5. New AuAg-Zn/MCM-36 catalyst - surface properties and catalytic activity/selectivity in methanol oxidation
    Authors:
    Iveta Kaskow, Anna Wojtaszek-Gurdak, Izabela Sobczak, Chia-Min Yang, Maria Ziolek
    Conference:
    XXII Zeolite Forum (rok: 2018, ), Wydawca: ISBN 978-83-950918-0-3
    Data:
    konferencja 19-23.06
    Status:
    Published
  6. Porous calcium oxides characterization and activity in transesterification processes
    Authors:
    D. Kryszak, M. Trejda
    Conference:
    XXII Zeolite Forum (rok: 2018, ), Wydawca: ISBN 978-83-950918-0-3
    Data:
    konferencja 19-23.06
    Status:
    Published
  7. The click chemistry re action as a tool for the generation of acid Or Basic center on mesoporous silicas and metallosilicates
    Authors:
    K. Stawicka, K. Drazkiewicz, V. Calvino-Casilda, R. Martin-Aranda, M. Ziolek
    Conference:
    7th FEZA Conference (rok: 2017, ), Wydawca: Uniwersytet w Sofii
    Data:
    konferencja 3-7.07
    Status:
    Published
  8. The creation of base catalysts by modification of SBA-15 and MCF mesoporous silicas by imidazole
    Authors:
    D. Kryszak, K. Stawicka, M. Trejda, M. Ziółek
    Conference:
    XLVIII Ogólnopolskie Kolokwium Katalityczne (rok: 2016, ), Wydawca: ISBN 978-83-60514-24-5
    Data:
    konferencja 16 - 18. 03
    Status:
    Published
  9. The generation of acidic and basic centers on mesoporous molecular sieves by click chemistry
    Authors:
    K. Stawicka, K. Drazkiewicz, V. Calvino-Casilda, R. M. Martin-Aranda
    Conference:
    XXI Forum Zeolitowe (rok: 2017, ), Wydawca: ISBN: 678-83-62783-10-6
    Data:
    konferencja 7-11.02
    Status:
    Published
  10. The impact of niobium and cerium on the basicity of calcium containing MCF materials
    Authors:
    Kalina Grzelak, Maciej Trejda, Maria Ziółek
    Conference:
    International Conference on Catalysis and Surface Chemistry (rok: 2018, ), Wydawca: ISBN 978-83-60514-28-3
    Data:
    konferencja 18-23.03
    Status:
    Published
  11. The role of phosphazene structure and cerium dopant on Basic properties of modified mesoporous cellular foams
    Authors:
    K. Stawicka, A. Klonowska, V. Calvino-Casilda, R. Martin-Aranda, M. Ziolek
    Conference:
    7th FEZA Post-Conference School (rok: 2017, ), Wydawca: Uniwersytet w Sofii
    Data:
    konferencja 7-9.07
    Status:
    Published
  12. AuCu-SBA-15 and AuCu-Nb/SBA-15 catalysts – the effect of niobium and support structure on activity in propene oxidation
    Authors:
    K. Grzelak, C-M. Yang, I. Sobczak, M. Ziolek
    Conference:
    Gold 2018 Conference, Paris (rok: 2018, ), Wydawca: xxx
    Data:
    konferencja 15-18.07
    Status:
    Published
  13. Ca/MCF doped with Nb and Ce as catalysts for transesterification of ethyl butyrate with methanol
    Authors:
    K. Grzelak, M. Trejda, M. Ziolek
    Conference:
    XXII Zeolite Forum (rok: 2018, ), Wydawca: ISBN 978-83-950918-0-3
    Data:
    konferencja 19-23.06
    Status:
    Published
  14. Modification of MWW zeolites in order to obtain new heterogeneous catalysts
    Authors:
    A. Wojtaszek-Gurdak
    Conference:
    XXI Forum Zeolitowe (rok: 2017, ), Wydawca: ISBN: 678-83-62783-10-6
    Data:
    konferencja 7-11.02
    Status:
    Published
  15. Modification of layered MWW zeolites by pillaring with niobium silicate
    Authors:
    A. Wojtaszek-Gurdak, M. Zielinska, M. Trejda, M. Ziolek
    Conference:
    18th International Zeolite Conference (rok: 2016, ), Wydawca: Uniwersytet w Rio de Janeiro
    Data:
    konferencja 19 - 24. 06
    Status:
    Published
  16. New modification routes of layered MWW zeolites by including niobium and amine species
    Authors:
    A. Wojtaszek-Gurdak, J. Latańska, M. Zagaja, M. Ziolek
    Conference:
    9th International Symposium on Group Five Elements (rok: 2017, ), Wydawca: Indian Institute of Technology, Kanpur
    Data:
    konferencja 22-24.11
    Status:
    Published
  17. Probing of basicity of MCFs modified with different nitrogen containing compounds with azastilbene
    Authors:
    K. Stawicka, D. Prukała, T. Siodła, M. Sikorski, M. Ziolek
    Conference:
    XXII Zeolite Forum (rok: 2018, ), Wydawca: ISBN 978-83-950918-0-3
    Data:
    konferencja 19-23.06
    Status:
    Published
  18. Search for the role of niobium component of molecular sieves in enhancement of catalytic activity
    Authors:
    M. Ziolek
    Conference:
    XX Zeolite Forum (rok: 2015, ), Wydawca: ISBN 978-83-929430-9-9
    Data:
    konferencja 22-26. 09
    Status:
    Published
  19. Fascinating niobium catalysts
    Authors:
    Maria Ziółek
    Conference:
    International Conference on Catalysis and Surface Chemistry (rok: 2018, ), Wydawca: ISBN 978-83-60514-28-3
    Data:
    konferencja 18-23.03
    Status:
    Published
  20. Generation of basicity in MWW zeolites towards the formation of bifunctional catalysts
    Authors:
    A. Wojtaszek-Gurdak, J. Latanska, M. Zagaja, M. Ziolek
    Conference:
    7th FEZA Conference (rok: 2017, ), Wydawca: Uniwersytet w Sofii
    Data:
    konferencja 3-7. 07
    Status:
    Published
  21. Mezopoorowate krzemionki i niobokrzemiany modyfikowane imidazolem - katalizatory zasadowe
    Authors:
    D. Kryszak, K. Stawicka, V. Calvino-Casilda, R. Martin Aranda, M. Ziółek
    Conference:
    59. Zjazd Naukowy Polskiego Towarzystwa Chemicznego (rok: 2016, ), Wydawca: ISBN 978-83-60988-23-7
    Data:
    konferencja 19 - 23. 09
    Status:
    Published
  22. Mezoporowate materiały typu SBA-15 modyfikowane wapniem i niobem - katalizatory zasadowe
    Authors:
    M. Trejda, E. Drgas, A. Zdziabek, M. Ziółek
    Conference:
    59. Zjazd Naukowy Polskiego Towarzystwa Chemicznego (rok: 2016, ), Wydawca: ISBN 978-83-60988-23-7
    Data:
    konferencja 19 - 23. 09
    Status:
    Published
  23. Modification of APTMS-Nb/MCF basicity by gold and copper dopants
    Authors:
    I. Sobczak, M. Wlodarczyk, L. Wolski, M. Ziolek, V. Calvino-Casilda, R. Martin-Aranda
    Conference:
    9th International Symposium on Group Five Elements (rok: 2017, ), Wydawca: Indian Institute of Technology, Kanpur
    Data:
    konferencja 22-24.11
    Status:
    Published
  24. The effect of niobium as a component of catalysts on the oxidation processes towards the production of fine chemicals
    Authors:
    M. Ziolek, I. Sobczak
    Conference:
    11th International Congress on Catalysis and Fine Chemicals (rok: 2016, ), Wydawca: Uniwersytet w Lyonie
    Data:
    konferencja 05 - 08. 09
    Status:
    Published
  25. The mobility of metallic species in Ce-Zr-oxides modified with Au and Cu and their catalytic performance in methanol oxidation
    Authors:
    P. Kamiński, M. Ziółek
    Conference:
    XLVIII Ogólnopolskie Kolokwium Katalityczne (rok: 2016, ), Wydawca: ISBN 978-83-60514-24-5
    Data:
    konferencja 16 - 18. 03
    Status:
    Published
  26. The synthesis of basic silicas and niobiosilicates SBA-15 and MCF by imidazole anchoring
    Authors:
    D. Kryszak, K. Stawicka, V. Calvino-Casilda, R.M. Martin-Aranda, M. Ziolek
    Conference:
    XXI Forum Zeolitowe (rok: 2017, ), Wydawca: ISBN: 678-83-62783-10-6
    Data:
    konferencja 7-11.02
    Status:
    Published
  27. Acid-base modification of layered MWW zeolites
    Authors:
    Anna Wojtaszek-Gurdak, Joanna Latańska, Marzena Zagaja, Aneta Grzesińska, Maria Ziółek
    Conference:
    International Conference on Catalysis and Surface Chemistry (rok: 2018, ), Wydawca: ISBN 978-83-60514-28-3
    Data:
    konferencja 18 - 23. 03
    Status:
    Published
  28. Ca/MCF materials – the impact of niobium on the basicity
    Authors:
    M. Trejda, D. Kryszak, N. Benedyczak, M. Ziolek
    Conference:
    9th International Symposium on Group Five Elements (rok: 2017, ), Wydawca: Indian Institute of Technology, Kanpur
    Data:
    konferencja 22-14.11
    Status:
    Published
  29. Generation of basic centers in mesoporous silicas and metallosilicates
    Authors:
    D. Kryszak. K. Stawicka, M. Trejda. V. Calvino-Casilda, R. Martin-Aranda, M. Ziolek
    Conference:
    7th FEZA Post-Conference School (rok: 2017, ), Wydawca: Uniwersytet w Sofii
    Data:
    konferencja 7-9.07
    Status:
    Published
  30. Gold-silver catalysts based on ZnO in propene oxidation – the effect of silver dopant and hydrogen treatment on catalytic properties
    Authors:
    Iveta Kaskow, C-M. Yang, I. Sobczak, M. Ziolek
    Conference:
    Gold 2018 Conference, Paris (rok: 2018, ), Wydawca: xxx
    Data:
    konferencja 15-18.07
    Status:
    Published
  31. Insight into the properties of calcium containing mesostructured cellular foams
    Authors:
    M. Trejda, N. Benedyczak, D. Kryszak
    Conference:
    7th FEZA Conference (rok: 2017, ), Wydawca: Uniwersytet w Sofii
    Data:
    konferencja 3-7.07
    Status:
    Published
  32. The effect of niobium and tantalum on physicochemical and catalytic properties of silver and platinum catalysts based on MCF mesoporous cellular foams
    Authors:
    J. Wisniewska, M. Ziolek, N. Artioli, M. Daturi
    Conference:
    The 16th International Congress on Catalysis (rok: 2016, ), Wydawca: Uniwersytet w Pekinie
    Data:
    konferencja 03 - 08. 07
    Status:
    Published
  33. The role of cerium and niobium species in base-acid properties of MCFs
    Authors:
    Katarzyna Stawicka, Piotr Decyk, Anna Wojtaszek-Gurdak, Maria Ziółek
    Conference:
    International Conference on Catalysis and Surface Chemistry (rok: 2018, ), Wydawca: ISBN 978-83-60514-28-3
    Data:
    konferencja 18-23.03
    Status:
    Published
  1. Gold Loaded on Niobium, Zinc and Cerium Oxides Synthesis, Characterization and Catalytic Application
    Authors:
    Maria Ziolek, Izabela Sobczak, Lukasz Wolski
    Book:
    Nanocatalysis Applications and Technologies (rok: 2019, tom: xx, strony: 254-299), Wydawca: CRC Press Taylor & Francis Group
    Status:
    Published
  2. Structure and reactivity of zeolites containing group five elements (V, Nb, Ta)
    Authors:
    M. Ziolek, I. Sobczak,m M. Trejda, A. Wojtaszek - Gurdak
    Book:
    Structure and Reactivity of Metals in Zeolite Materials in Series: Structure and Bonding (rok: 2018, tom: 178, strony: 179-251), Wydawca: Springer
    Status:
    Published