Projects funded by the NCN

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Principal investigator

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Information of the project and the call

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Platinum Group Organometallics Based on Carbaporphyrinoids: Pursuit for New Generation of Functional Modules

2012/04/A/ST5/00593

Keywords:

carbaporphyrinoid platinum group metals porphyrin aromaticity molecular devices catalysis

Descriptors:

ST5_23:
ST5_14:
ST5_9:

Panel:

ST5 - Materials: materials synthesis, structure-properties relations, advanced and functional materials with designed properties, (macro)molecular architecture, material engineering

Host institution :

Uniwersytet Wrocławski, Wydział Chemii

woj. dolnośląskie

Other projects carried out by the institution

Principal investigator (from the host institution):

prof. Cyryl Lechosław Latos-Grażyński

Number of co-investigators in the project: 14

Call: MAESTRO 2 - announced on 2011-12-15

Amount awarded: 2 997 400 PLN

Project start date (Y-m-d): 2012-09-17

Project end date (Y-m-d): 2018-09-16

Project duration:: 72 months (the same as in the proposal)

Project status: Project settled

Equipment purchased [PL]

Komora rękawicowa wyposażona w lodówkę i zestaw odpowiednich śluz (255 000 PLN)
Pompa membranowe 2x17500 (2 szt.) (35 000 PLN)
Zestaw: mieszadło z płytą ceramiczną i kontaktowym termometrem (6 szt.) (12 000 PLN)
Aparatura HPLC (skala półpreparatywna) zaopatrzona w kolektor frakcji, detector UV-vis i preparatywny autosampler (250 000 PLN)
Równoległa stacja robocza do zastosowań syntetycznych w fazie ciekłej i stałej wyposażona w system podgrzewania/chłodzenia (86 000 PLN)
Pompa strzykawkowa.
Spektrofluorometer z detekcją powyżej 1000 nm-1 (120 000 PLN)
Wyparki rotacyjne z pionowym zestawem chłodnic (2 szt.) (32 000 PLN)
Pompa do linii próżniowych (3 szt.) (45 000 PLN)
Cyrkulator chłodzący (33 000 PLN)
System próżniowy.

Information in the final report

Publication in academic press/journals (48)

Core chemistry and skeletal rearrangements of porphyrinoids and metalloporphyrinoids.
Authors:
Szyszko, B.; Latos-Grażyński, L.
Academic press:
Chem. Soc. Rev. (rok: 2015, tom: 44, strony: 3588-3616), Wydawca: RSC
Status:
Published
DOI:
10.1039/c4cs00398e - link to the publication
Fused Meso-Aminoporphyrin: A Switchable Near-IR Chromophore.
Authors:
Pawlicki M., Hurej K., Kwiecińska K., Szterenberg L., Latos-Grażyński L.
Academic press:
Chem.Comm. (rok: 2015, tom: 51, strony: 11362-11365), Wydawca: RSC
Status:
Published
DOI:
10.1039/c5cc01231g - link to the publication
Palladium(II), Ruthenium(II) and Ruthenium(III) Complexes of 23-thiaazuliporphyrin. The case of coordination-induced contraction.
Authors:
Białek, M.; Latos-Grażyński, L.
Academic press:
Inorg. Chem. (rok: 2016, tom: 55, strony: 1758-1769.), Wydawca: ACS
Status:
Published
DOI:
10.1021/acs.inorgchem.5b02684 - link to the publication
Tweezing: Ruthenium Clusters Docked at Azuliporphyrinogens
Authors:
Białek,M.; Sprutta,N; Latos-Grażyński,L.
Academic press:
Inorg.Chem. (rok: 2016, tom: 56, strony: 12061-12073), Wydawca: ACS
Status:
Published
DOI:
10.1021/acs.inorgchem.6b02228 - link to the publication
Photooxidation of Unhindered Triarylcorroles.
Authors:
Wojaczyński, J.; Duszak, M.; Latos-Grażyński, L.
Academic press:
Tetrahedron (rok: 2013, tom: 69, strony: 10445-10449), Wydawca: Elsevier
Status:
Published
DOI:
10.1016/j.tet.2013.09.090 - link to the publication
A Porphyrin Skeleton Containing a Palladacyclopentadiene.
Authors:
Pacholska-Dudziak, E.; Szczepaniak, M.; Książek, A.; Latos-Grażyński, L
Academic press:
Angew. Chem. Int. Ed. (rok: 2013, tom: 52, strony: 8898-8903), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/anie.201304493 - link to the publication
Möbius-Hückel Topology Switching in an Expanded Porphyrin Cation Radical as Studied by EPR and ENDOR Spectroscopy.
Authors:
Möbius, K.; Plato, M.; Klihm, G.; Laurich, C.; Savitsky, A.; Lubitz, W.; Szyszko, B.; Stępień, M.;
Academic press:
Phys.Chem.Chem.Phys. (rok: 2015, tom: 17, strony: 644-652), Wydawca: Royal Society of Chemistry
Status:
Published
DOI:
10.1039/c4cp05745g - link to the publication
Helicenophyrins - Expanded Carbaporphyrins Incorporating Aza[5]Helicene and Heptacyclic S-Shaped Aza[5]Helicene Motifs
Authors:
Szyszko, B.; Przewoźnik, M.; Białek, M.; Białońska, A.; Cichosz, J.; Latos-Grażyński, L.
Academic press:
Angew. Chem., Int. Ed. (rok: 2018, tom: 57, strony: 4030-4034), Wydawca: Wiley - VCH
Status:
Published
DOI:
10.1002/anie.201800879 - link to the publication
A Three Stage Aromaticity Switching in Boron(III) and Phosphorus(V) N-Fused p-Benziporphyrin.
Authors:
Idec, A.; Pawlicki, M.; Latos-Grażyński, L.
Academic press:
Chem.Eur.J. (rok: 2019, tom: 25, strony: 200 – 204), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/chem.201804983 - link to the publication
Triggered Transformations of 22-Methyl-m-Benziporphyrin Involving an Effective Contraction of Benzene to Cyclopentadiene.
Authors:
Hurej, K.; Pawlicki, M.; Latos-Grażyński
Academic press:
Chem.Eur.J. (rok: 2017, tom: 23, strony: 2509-2066), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/chem.201604458 - link to the publication
Rhodium-Induced Reversible C-C Bond Cleavage - Transformations of Rhodium(III) 22-Alkyl-m-Benziporphyrins
Authors:
Hurej,K.;Pawlicki, M.; Latos-Grażyński, L.
Academic press:
Chem. Eur. J. (rok: 2018, tom: 23, strony: 115-126), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/chem.201704411 - link to the publication
Oxidation and Oxygenation of Carbonyl Ruthenium(II) Azuliporphyrin.
Authors:
Białek, M.; Białońska, A.; Latos-Grażyński, L.
Academic press:
Inorg. Chem. (rok: 2015, tom: 54, strony: 6184-6194.), Wydawca: ACS
Status:
Published
DOI:
10.1021/acs.inorgchem.5b00324 - link to the publication
Oxatriphyrins(2.1.1) Incorporating ortho-Phenylene Motif
Authors:
Pawlicki M.; Garbicz M.; Latos-Grazyński L.
Academic press:
Angew. Chem. Int. Ed. (rok: 2015, tom: 54, strony: 1906 –1909), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/anie.201410595 - link to the publication
Aromaticity Switching Via Azulene Transformations in Azulene-Bridged A,D-Dithiahexaphyrin
Authors:
Białek, M.J.; Latos-Grażyńsk,i L.
Academic press:
Chem. Comm. (rok: 2018, tom: 54, strony: 1837-1840), Wydawca: Royal Society of Chemistry
Status:
Published
DOI:
10.1039/c7cc08754c - link to the publication
Flexible porphyrinoids
Authors:
Szyszko,B.; Białek,M.; Pacholska-Dudziak,E.; Latos-Grażyński,L.
Academic press:
Chem.Rev. (rok: 2017, tom: 117, strony: 2839-2909), Wydawca: ACS
Status:
Published
DOI:
10.1021/acs.chemrev.6b00423 - link to the publication
Ruthenium(II) and Ruthenium(III) Complexes of p-Benziporphyrin: Merging Equatorial and Axial Organometallic Coordination
Authors:
Idec, A.; Pawlicki, M.;Latos-Grażyński, L.
Academic press:
Inorganic Chemistry (rok: 2017, tom: 56, strony: 10337-10352), Wydawca: American Chemical Society
Status:
Published
DOI:
10.1021/acs.inorgchem.7b01237 - link to the publication
Gold(III) Mediated Contraction of Benzene to Cyclopentadiene: From P-Benziporphyrin to Gold(III) True Tetraarylcarbaporphyrin.
Authors:
Szyszko, B.; Kupietz, K.; Szterenberg, L.; Latos-Grażyński, L.
Academic press:
Chem.Eur.J. (), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/chem.201304162 - link to the publication
Inversion Triggered by Protonation - A Rubyrin With an Embedded a,b'-Pyridine Moieties.
Authors:
Myśliborski, R.; Hurej, K.; Pawlicki, M.; Latos-Grażyński, L.
Academic press:
Angew. Chem. Int. Ed. (), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/anie.201811138 - link to the publication
Aromaticity Switching Via Azulene Transformations in Azulene-Bridged A,D-Dithiahexaphyrin
Authors:
Białek, M.J.; Latos-Grażyńsk,i L.
Academic press:
Chem. Comm. (), Wydawca: Royal Society of Chemistry
Status:
Published
DOI:
10.1039/c7cc08754c - link to the publication
A Mixed Valence Bis-Phosphorus Complex Entrapped in the Oxatriphyrin(3.1.1) Surrounding
Authors:
Idec,A.; Skonieczny,J.; Latos-Grażyński,L.; Pawlicki,M.
Academic press:
Eur.J.Org.Chem. (rok: 2016, tom: 2016, strony: 3691-3695), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/ejoc.201600701 - link to the publication
Phenanthriporphyrin: Antiaromatic Aceneporphyrinoid as Surrounding for Hypervalent Organophosphorus(V).
Authors:
Szyszko, B.; Szterenberg, L.; Białońska, A.; Latos-Grażyński, L.
Academic press:
Angew. Chem. Int. Ed. (rok: 2015, tom: 54, strony: 4932-4936), Wydawca: Wiley VCH
Status:
Published
DOI:
10.1002/anie.201500732 - link to the publication
Incorporation of Phenanthrene Subunit into Sapphyrin Framework - Toward Expanded Aceneporphyrinoids
Authors:
Szyszko,B.; Małecki,M.; Berlicka,A.; Białek,M.J.; Białońska,A.; Kupietz,K.; Pacholska-Dudziak,E.; Latos-Grażyński,L.
Academic press:
Chem.Eur.J. (rok: 2016, tom: 22, strony: 7602-7608), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/chem.201600606 - link to the publication
Incorporation of 1,5-Naphthalene Subunit into Heteroporphyrin Structure - Toward Helical Aceneporphyrinoids
Authors:
Szyszko, B.; Pacholska-Dudziak, E.; Latos-Grażyński, L.
Academic press:
J. Org. Chem. (rok: 2013, tom: 78, strony: 5090-5095), Wydawca: ACS
Status:
Published
DOI:
10.1021/jo4006624 - link to the publication
Merging of inner and outer ruthenium organometallic coordination motifs within an azuliporphyrin framework.
Authors:
Białek M. J., Latos-Grażyński L.
Academic press:
Chem.Comm. (rok: 2014, tom: 50, strony: 9270-9272), Wydawca: The Royal Society of Chemistry
Status:
Published
DOI:
0.1039/c4cc04271a - link to the publication
Toward True Carbaporphyrinoids: Synthesis of 21-Carba-23-Thiaporphyrin.
Authors:
Berlicka, A.; Dutka, P.; Szterenberg, L.; Latos-Grażyński, L.
Academic press:
Angew. Chem. Int. Ed. (rok: 2014, tom: 53, strony: 4485-4489), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/anie.201310999 - link to the publication
meso-Tetraaryl-21-carbaporphyrin - Incorporation of a Cyclopentadiene Unit into a Porphyrin Architecture
Authors:
Garbicz,M.; Latos-Grażyński,L.
Academic press:
Angew.Chem.Int.Ed. (rok: 2019, tom: 58, strony: 6089-6093), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/anie.201901808 - link to the publication
Retrieving Aromaticity of Dithiadiazuliporphyrin by oxidation: Illustration by Experimental and Theoretical Investigation .
Authors:
Sung, Y. M.; Sprutta, N.; Kim, J. O.; Koo, Y. H.; Latos-Grażyński, L.; Kim, D.
Academic press:
RSC Advances (rok: 2017, tom: 7, strony: 19502-19505), Wydawca: Royal Society of Chemistry
Status:
Published
DOI:
10.1039/c7ra02458d - link to the publication
Aromaticity Switching in Porphyrinoids.
Authors:
Pawlicki, M.; Latos-Grażyński, L.
Academic press:
Chem. Asian J. (rok: 2015, tom: 10, strony: 1438-1451), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/asia.201500170 - link to the publication
A parallel-displaced directly linked 21-carba-23-thiaporphyrin dimer incorporating a dihydrofulvalene motif
Authors:
Berlicka,A.; Białek,M.; Latos-Grażyński,L.
Academic press:
Angew.Chem.Int.Ed. (rok: 2016, tom: 55, strony: 11231-11236), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/anie.201606298 - link to the publication
Hückel and Möbius Expanded Porphyrins:Synthesis and Aromaticity Switching
Authors:
Szyszko, B.; Sprutta, N.; Chwalisz, P.; Stępień, M.; Latos-Grażyński, L
Academic press:
Chem. Eur.J. (rok: 2014, tom: 20, strony: 1985–1997), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/chem.201304162 - link to the publication
L-Proline catalyzed reaction of N-confused porphyrin and active methylene compounds
Authors:
B. Liu, X. Li,. J. Zhang, P. J. Chmielewski
Academic press:
Org.Biomol.Chem. (rok: 2013, tom: 11, strony: 4831-4839), Wydawca: RSC
Status:
Published
DOI:
10.1039/c3ob40754c - link to the publication
Organocopper(III) Phenanthriporphyrin – Exocyclic Transformations
Authors:
Kupietz,K.; Białońska,A.; Szyszko,B.; Latos-Grażyński,L.
Academic press:
Inorg.Chem. (rok: 2019, tom: 58, strony: 1451-1461), Wydawca: ACS
Status:
Published
DOI:
10.1021/acs.inorgchem.8b02997 - link to the publication
The effect of pi-conjugation in the macrocyclic in the macrocyclic ring on the photophysical properties of a series of thiaaceneporphyrinoids
Authors:
Sung Y.M, Szyszko B., Radomir MyśliborskiR., Stępień M., Oh J.,Son M.,Latos-Grażyński L., Kim D.
Academic press:
Chem. Commun. (), Wydawca: The Royal Society of Chemistry
Status:
Published
DOI:
10.1039/c4cc03855j - link to the publication
meso-Tetraaryl-21-carbaporphyrin - Incorporation of a Cyclopentadiene Unit into a Porphyrin Architecture
Authors:
Garbicz,M.; Latos-Grażyński,L.
Academic press:
Angew.Chem.Int.Ed. (), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/anie.201901808 - link to the publication
L-Proline catalyzed reaction of N-confused porphyrin and active methylene compounds
Authors:
B. Liu, X. Li,. J. Zhang, P. J. Chmielewski
Academic press:
Org.Biomol.Chem. (), Wydawca: RSC
Status:
Published
DOI:
10.1039/c3ob40754c - link to the publication
From para benziporphyrin to rhodium(III) 21-carbaporphyrins : imprinting Rh···η2-CC, Rh···η2-CO, and Rh···η2-CH coordination motifs.
Authors:
Idec A., Szterenberg L., Latos-Grażyński L.
Academic press:
Chem.Eur.J., (rok: 2015, tom: 21, strony: 12481-12487), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/chem.201501996 - link to the publication
A Rhodium Mediated Contraction of Benzene to Cyclopentadiene. Transformations of Rhodium(III) m-Benziporphyrin.
Authors:
Hurej, K.; Pawlicki, M.; Szterenberg, L.; Latos-Grażyński, L.
Academic press:
Angew. Chem. Int. Ed. (rok: 2016, tom: 55, strony: 1427-1431), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/anie.201508033 - link to the publication
Meso-N-Pyrrole As a Versatile Substituent Influencing the Optical Properties of Porphyrin.
Authors:
Hurej,K.; Stawski,W.; Latos-Grażyński,L.; Pawlicki,M.
Academic press:
Chem.Asian.J. (rok: 2016, tom: 11, strony: 329-333), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/asia.201601210 - link to the publication
Gold(III) Mediated Contraction of Benzene to Cyclopentadiene: From P-Benziporphyrin to Gold(III) True Tetraarylcarbaporphyrin.
Authors:
Szyszko, B.; Kupietz, K.; Szterenberg, L.; Latos-Grażyński, L.
Academic press:
Chem.Eur.J. (rok: 2014, tom: 20, strony: 1376-1382), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/chem.201304162 - link to the publication
Ruthenocenoporphyrinoids - Conformation Determines Macrocyclic pi-Conjugation Transmitted Across a d-Electron Metallocene.
Authors:
Grocka, I.; Latos-Grażyński, L.; Stępień, M.
Academic press:
Angew. Chem. Int. Ed. 2013, 52, 1044-1048. (rok: 2013, tom: 52, strony: 1044-1048), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/anie.201208289 - link to the publication
Reversible reduction of oxatriphyrin(3.1.1)—adjusting the coordination abilities to the central ion.
Authors:
Pawlicki M., Kędzia A., Bykowski D., Latos-Grażyński L.
Academic press:
Chem.Eur.J. (rok: 2014, tom: 20, strony: 17500-17506), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/chem.201404570 - link to the publication
Synthesis and Switching the Aromatic Character of Oxatriphyrins(2.1.1).
Authors:
Pawlicki, M.; Hurej, K.; Szterenberg, L.; Latos-Grażyński, L.
Academic press:
Angew. Chem. Int. Ed. (rok: 2014, tom: 53, strony: 2992-2996), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/anie.201310129 - link to the publication
The effect of pi-conjugation in the macrocyclic in the macrocyclic ring on the photophysical properties of a series of thiaaceneporphyrinoids
Authors:
Sung Y.M, Szyszko B., Radomir MyśliborskiR., Stępień M., Oh J.,Son M.,Latos-Grażyński L., Kim D.
Academic press:
Chem. Commun. (rok: 2014, tom: 50, strony: 8367-8369), Wydawca: The Royal Society of Chemistry
Status:
Published
DOI:
10.1039/c4cc03855j - link to the publication
Incorporation of p-Phenylene Unit into the Azuliporphyrinogens Frame - Oxidation and Ruthenium Cluster Coordination
Authors:
Sprutta, N.; Hassa, A.; Białek, M. J.; Kodź-Wichowska, K.; Kupietz, K.; Latos-Grażyński, L.
Academic press:
Chem.Eur.J. (rok: 2018, tom: 23, strony: 14686-14692), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/chem.201802972 - link to the publication
Inversion Triggered by Protonation - A Rubyrin With an Embedded a,b'-Pyridine Moieties.
Authors:
Myśliborski, R.; Hurej, K.; Pawlicki, M.; Latos-Grażyński, L.
Academic press:
Angew. Chem. Int. Ed. (rok: 2019, tom: 57, strony: 16866-16870), Wydawca: Wiley-VCH
Status:
Published
DOI:
10.1002/anie.201811138 - link to the publication
Oxygenation of Phenanthriporphyrin and Copper(III) Phenanthriporphyrin - An Efficient Route to Phenanthribilinones.
Authors:
Kupietz, K.; Białek, M. J.; Hassa, K.; Białońska, A.; Latos-Grażyński, L.
Academic press:
Inorg.Chem. (rok: 2019, tom: 58, strony: 12446-12456), Wydawca: ACS
Status:
Published
DOI:
10.1021/acs.inorgchem.9b02183 - link to the publication
Carbocations confined in a thiatriazuliporphyrin frame
Authors:
Sprutta,N.; Wełnic,M.; Białek,M.; Lis,T.; Szterenberg,L.; Latos-Grażyński,L.
Status:
Accepted for publication
Aromaticity Control via Modifications of a Macrocyclic Frame: 5,6-Dimethoxyphenanthriporphyrin and 5,6-Dioxophenanthri-porphyrin
Authors:
Kupietz, K.;Białek, J.J.;Białońska,A.;Szyszko,B.;Latos-Grażyński,L.
Status:
Accepted for publication

Information on the principal investigator and host institution

Information of the project and the call

Keywords

Equipment

Platinum Group Organometallics Based on Carbaporphyrinoids: Pursuit for New Generation of Functional Modules

Equipment purchased [PL]

Information in the final report

O Narodowym Centrum Nauki

Finansowanie nauki

Współpraca zagraniczna

Centrum prasowe

Partnerzy

Search form

Projects funded by the NCN

Information on the principal investigator and host institution

Information of the project and the call

Keywords

Equipment

Platinum Group Organometallics Based on Carbaporphyrinoids: Pursuit for New Generation of Functional Modules

Equipment purchased [PL]

Information in the final report

O Narodowym Centrum Nauki

Finansowanie nauki

Współpraca zagraniczna

Centrum prasowe

Partnerzy