Projects funded by the NCN

Information on the principal investigator and host institution

Information of the project and the call

Keywords

Equipment

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Multifunctional catalysts for the production of carboxylic acids from the renewable sources

2018/29/B/ST5/00137

Keywords:

Acid-redox catalysts zeolites mesoporous materials charcteristic oxidation of glucose oxidehydration of glycerol tandem oxidehydration of ethanol

Descriptors:

  • ST5_3: Surface modification
  • ST5_6: Porous materials, ceramics, glasses
  • ST5_18:

Panel:

ST5 - Materials: materials synthesis, structure-properties relations, advanced and functional materials with designed properties, (macro)molecular architecture, material engineering

Host institution :

Uniwersytet im. Adama Mickiewicza w Poznaniu, Wydział Chemii

woj. wielkopolskie

Other projects carried out by the institution 

Principal investigator (from the host institution):

prof. Maria Ziółek 

Number of co-investigators in the project: 9

Call: OPUS 15 - announced on 2018-03-15

Amount awarded: 1 904 400 PLN

Project start date (Y-m-d): 2019-01-10

Project end date (Y-m-d): 2023-01-09

Project duration:: 48 months (the same as in the proposal)

Project status: Project settled

Project description

Download the project description in a pdf file

Note - project descriptions were prepared by the authors of the applications themselves and placed in the system in an unchanged form.

Equipment purchased [PL]

  1. Rotor do wirówki.
  2. Wirówka.
  3. Auto-sampler do reaktora cieczowego Easy Max (140 000 PLN)
  4. Regulatory masowego przepływu.
  5. Reaktor - kuweta IR.
  6. Spektrometr INVENIO-S Fourier Transform Infrared.
  7. Chromatograf cieczowy HPLC (300 000 PLN)
  8. Kriostat.

Information in the final report

  • Publication in academic press/journals (17)
  • Articles in post-conference publications (21)
  • Book publications / chapters in book publications (1)
  1. Gold-containing Beta zeolite in base-free glucose oxidation – The role of Au deposition procedure and zeolite dopants
    Authors:
    Joanna Wolska, Adrian Walkowiak, Izabela Sobczak, Lukasz Wolski, Maria Ziolek
    Academic press:
    Catalysis Today (rok: 2021, tom: 382, strony: 48-60), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.cattod.2021.05.020 - link to the publication
  2. The impact of Ce/Nb dopant ratio on basicity of MCF modified with calcium species
    Authors:
    Kalina Grzelak, Maria Ziolek, Maciej Trejda
    Academic press:
    Catalysis Communications (rok: 2020, tom: 142, strony: 106045), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.catcom.2020.106045 - link to the publication
  3. The importance of residual water for the reactivity of MPTMS with silica on the example of SBA-15
    Authors:
    Katarzyna Stawicka, Maciej Gierada, Julia Gajewska, Frederik Tielens, Maria Ziolek
    Academic press:
    Applied Surface Science (rok: 2020, tom: 513, strony: 145802), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.apsusc.2020.145802 - link to the publication
  4. Calcium and nitrogen species loaded into SBA-15 – a promising catalyst tested in Knoevenagel condensation
    Authors:
    Dorota Kryszak, Katarzyna Stawicka, Maciej Trejda
    Academic press:
    Dalton Transactions (rok: 2020, tom: 49, strony: 9781), Wydawca: Royal Society of Chemistry
    Status:
    Published
    DOI:
    10.1039/d0dt01621g - link to the publication
  5. Activation of ethanol transformation on copper-containing SBA-15 and MnSBA-15 catalysts by the presence of oxygen in the reaction mixture
    Authors:
    Izabela Sobczak, Joanna Wisniewska, Piotr Decyk, Maciej Trejda and Maria Ziolek
    Academic press:
    International Journal of Molecular Sciences (rok: 2023, tom: 24, strony: 2252), Wydawca: MDPI
    Status:
    Published
    DOI:
    brak - link to the publication
  6. Modification of Gold Zeolitic Supports for Catalytic Oxidation of Glucose to Gluconic Acid
    Authors:
    Adrian Walkowiak, Joanna Wolska, Anna Wojtaszek-Gurdak, Izabela Sobczak, Lukasz Wolski, Maria Ziolek
    Academic press:
    Materials (rok: 2021, tom: 14, strony: 5250), Wydawca: MDPI
    Status:
    Published
    DOI:
    10.3390/ma14185250 - link to the publication
  7. Niobium: The Focus on Catalytic Application in the Conversion of Biomass and Biomass Derivatives
    Authors:
    Luiz Oliveira, Márcio Pereira, Ana Pacheli Heitman, José Filho, Cinthia Oliveira and Maria Ziolek
    Academic press:
    Molecules (rok: 2023, tom: 28, strony: 1527), Wydawca: MDPI
    Status:
    Published
    DOI:
    10.3390/molecules28041527 - link to the publication
  8. The Impact of 3-(trihydroxysilyl)-1-propanesulfonic Acid Treatment on the State of Vanadium Incorporated on SBA-15 Matrix
    Authors:
    Ardian Nurvita, Piotr Decyk, Maria Ziolek, Maciej Trejda
    Academic press:
    Catalysts (rok: 2021, tom: 11, strony: 397), Wydawca: MDPI
    Status:
    Published
    DOI:
    10.3390/ - link to the publication
  9. Towards efficient acidic catalysts via optimization of SO3H-organosilane immobilization on SBA-15 under increased pressure – potential application in gas and liquid phase reactions
    Authors:
    Maciej Trejda, Ada Kaszuba, Ardian Nurwita and Maria Ziolek
    Academic press:
    Materials (rok: 2021, tom: 14, strony: 7226), Wydawca: MDPI
    Status:
    Published
    DOI:
    10.3390/ma14237226 - link to the publication
  10. A platinum promoted Ag/SBA-15 catalyst effective in selective oxidation of methanol – design and surface characterization
    Authors:
    Joanna Wisniewska, Izabela Dziedzic, Maria Ziolek
    Academic press:
    RSC Advances (rok: 2020, tom: 10, strony: 14570), Wydawca: Royal Society of Chemistry
    Status:
    Published
    DOI:
    10.1039/d0ra01562h - link to the publication
  11. Development of a method for the synthesis of basic catalysts with high number of active species
    Authors:
    Katarzyna Stawicka
    Academic press:
    Catalysis Today (rok: 2020, tom: 354, strony: 51-60), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.cattod.2019.09.013 - link to the publication
  12. Gold based on SBA-15 supports – Promising catalysts in base-free glucose oxidation
    Authors:
    Joanna Wisniewska, Izabela Sobczak, Maria Ziolek
    Academic press:
    Chemical Engineering Journal (rok: 2021, tom: 413, strony: 127548), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.cej.2020.127548 - link to the publication
  13. Insight into Active Centers and Anti-Coke Behavior of Niobium-Containing SBA-15 for Glycerol Dehydration
    Authors:
    Katarzyna Stawicka, Maciej Trejda, Maria Ziolek
    Academic press:
    Catalysts (rok: 2021, tom: 11, strony: 45309), Wydawca: MDPI
    Status:
    Published
    DOI:
    10.3390/catal11040488 - link to the publication
  14. The effect of the calcium dopant on the activity and selectivity of gold catalysts supported on SBA-15 and Nb-containing SBA-15 in methanol oxidation
    Authors:
    Joanna Wisniewska, Izabela Sobczak, Maria Ziolek
    Academic press:
    Catalysis Science & technology (rok: 2021, tom: 11, strony: 2242), Wydawca: Royal Society of Chemistry
    Status:
    Published
    DOI:
    10.1039/d0cy02135k - link to the publication
  15. Enhancement of selectivity in methanol oxidation over copper containing SBA-15 by doping with boron species
    Authors:
    Zih-Yi Yang, Anna Wojtaszek-Gurdak, Chia-Min Yang, Maria Ziolek
    Academic press:
    Catalysis Today (rok: 2020, tom: 356, strony: 122-131), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.cattod.2019.06.035 - link to the publication
  16. Microwave-Assisted Base-Free Oxidation of Glucose with H2O2 on Gold- and Manganese-Containing SBA-15—Insight into Factors Affecting the Reaction Pathway
    Authors:
    Izabela Sobczak, Tsering Chödon Kowalska, Magdalena Nowicka and Maria Ziolek
    Academic press:
    International Journal of Molecular Sciences (rok: 2022, tom: 23, strony: 4639), Wydawca: MDPI
    Status:
    Published
    DOI:
    10.3390/ijms23094639 - link to the publication
  17. The effect of support properties on n-octanol oxidation performed on gold – silver catalysts supported on MgO, ZnO and Nb2O5
    Authors:
    Iveta Kaskow, Izabela Sobczak, Maria Ziolek, Vicente Cortés Corberán
    Academic press:
    Molecular Catalysis (rok: 2020, tom: 482, strony: 110674), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.mcat.2019.110674 - link to the publication
  1. Base-free oxidation of glucose on Au/SBA-15 and Au/NbSBA-15 catalysts modified with calcium
    Authors:
    Joanna Wiśniewska, Angelika Wrublińska, Izabela Sobczak, Maria Ziółek
    Conference:
    LII Ogólnopolskie Kolokwium Katalityczne (rok: 2020, ), Wydawca: Kraków, Instytut Katalizy i Fizykochemii Powierzchni im. Jerzego Habera PAN
    Data:
    konferencja 25-27 XI
    Status:
    Published
  2. Influence of niobium and cerium dopants on optical and catalytic properties of gold catalysts supported on zeolite Beta
    Authors:
    Adrian Walkowiak, Joanna Wolska, Łukasz Wolski, Izabela Sobczak, Maria Ziółek
    Conference:
    LII Ogólnopolskie Kolokwium Katalityczne (rok: 2020, ), Wydawca: Kraków, Instytut Katalizy i Fizykochemii Powierzchni im. Jerzego Habera PAN
    Data:
    konferencja 25-27 XI
    Status:
    Published
  3. Microwave-assisted base-free oxidation of glucose with H2O2 on Au-MnSBA-15 and Cu-MnSBA-15 mesoporous sieves
    Authors:
    Izabela Sobczak, Tsering Kowalska, Magdalena Nowicka, Maria Ziolek
    Conference:
    Gold 2022 Conference; Quebeck City (rok: 2022, ), Wydawca: Organizing Commitee
    Data:
    konferencja 17-20 July 2022
    Status:
    Published
  4. Activity of MWW zeolites with different basic centers in Knoevenagel condensation
    Authors:
    Anna Wojtaszek-Gurdak, Vanesa Calvino-Casilda, Aneta Grzesinska, Rosa Martin-Aranda, Maria Ziolek
    Conference:
    14th EuropaCat - European Congress on Catalysis "Catalysis without Borders" (rok: 2019, ), Wydawca: Organizatorzy Konferencji - Kluby Katalizy: Niemcy, Holandia, Belgia
    Data:
    konferencja 18-23 sierpnia 2019
    Status:
    Published
  5. Insight into the factors affecting base-free glucose oxidation on gold-containing Beta zeolite – the role of Au deposition procedure and zeolite dopants
    Authors:
    J. Wolska, A. Walkowiak, I. Sobczak, L. Wolski, and M. Ziolek
    Conference:
    9th World Congress on Oxidation Catalysis: Oxidation for a Sustainable Future and Clean Environment; Cardiff (rok: 2022, ), Wydawca: Organizing Commitee
    Data:
    konferencja 4-8 September 2022
    Status:
    Published
  6. The effect of water on the efficiency of MPTMS anchoring and its stability in mesoporous silica SBA-15
    Authors:
    Katarzyna Stawicka, Julia Gajewska, Maciej Gierada, Christina Siakati, Frederik Tielens, Maria Ziolek
    Conference:
    14th EuropaCat - European Congress on Catalysis "Catalysis without Borders" (rok: 2019, ), Wydawca: Organizatorzy Konferencji - Kluby Katalizy: Niemcy, Holandia, Belgia
    Data:
    konferencja 18-23 sierpnia 2019
    Status:
    Published
  7. The impact of Au deposition method on the catalytic performance of Beta zeolite-based gold catalysts in base-free glucose oxidation
    Authors:
    A. Walkowiak, J. Wolska, I. Sobczak, L. Wolski, M. Ziolek
    Conference:
    8th Conference of the Federation of European Zeolite Associations (FEZA 2021) (rok: 2021, ), Wydawca: https://www.fezaconference.org/programme/virtual-programme-overview/
    Data:
    konferencja 5 - 9 lipca
    Status:
    Published
  8. The role of water in SBA-15 on efficiency of MPTMS and APTMS anchoring
    Authors:
    Katarzyna Stawicka, Maciej Gierada, Julia Gajewska, Frederik Tielens, Maria Ziolek
    Conference:
    LII Ogólnopolskie Kolokwium Katalityczne (rok: 2020, ), Wydawca: Kraków, Instytut Katalizy i Fizykochemii Powierzchni im. Jerzego Habera PAN
    Data:
    konferencja 25-27 XI
    Status:
    Published
  9. Bimetallic AuAg catalysts supported on MgO, ZnO and Nb2O5 for noctanol oxidation: the effect of support and preactivation
    Authors:
    Iveta Kaskow, Izabela Sobczak, Maria Ziolek, Vicente Cortez Corberan
    Conference:
    14th EuropaCat - European Congress on Catalysis "Catalysis without Borders" (rok: 2019, ), Wydawca: Organizatorzy Konferencji - Kluby Katalizy: Niemcy, Holandia, Belgia
    Data:
    konferencja 18-23 sierpnia 2019
    Status:
    Published
  10. Gold catalysts supported on 2D and 3D zeolites – characterization and application in base-free glucose oxidation
    Authors:
    Adrian Walkowiak, Joanna Wolska, Anna Wojtaszek-Gurdak, Izabela Sobczak, Lukasz Wolski, Maria Ziolek
    Conference:
    LIII Ogólnopolskie Kolokwium Katalityczne (rok: 2021, ), Wydawca: Powierzchni im. Jerzego Habera PAN
    Data:
    konferencja 22 - 24 września
    Status:
    Published
  11. The effect of calcium dopant in Au/SBA-15 and Au/NbSBA-15 on the catalytic properties in oxidation of glucose and methanol
    Authors:
    J. Wisniewska, I. Sobczak, M. Ziolek
    Conference:
    15th Pannonian International Symposium on Catalysis (rok: 2022, ), Wydawca: toteMedia Lublin, Poland
    Data:
    konferencja 4-8 September 2022
    Status:
    Published
  12. Wpływ metody wprowadzania Au na właściwości katalizatorów złotowych osadzonych na zeolicie Beta
    Authors:
    Adrian Walkowiak, Joanna Wolska, Izabela Sobczak, Łukasz Wolski, Maria Ziółek
    Conference:
    63. Zjazd naukowy Polskiego Towarzystwa Chemicznego (rok: 2021, ), Wydawca: PTChem
    Data:
    konferencja 13 - 16 września
    Status:
    Published
  13. Ce and Nb as dopants in Ca/MCF system for enhancement of basicity
    Authors:
    K. Grzelak, M. Trejda, M. Ziolek
    Conference:
    8th Conference of the Federation of European Zeolite Associations (FEZA 2021) (rok: 2021, ), Wydawca: https://www.fezaconference.org/programme/virtual-programme-overview
    Data:
    konferencja 5 - 9 lipca
    Status:
    Published
  14. In search for the best bifunctional catalysts, based on MnSBA-15 and modified with Cu or Au, addressed to oxydehydration of glycerol
    Authors:
    Izabela Sobczak, Magdalena Nowicka, Maria Ziółek
    Conference:
    LIII Ogólnopolskie Kolokwium Katalityczne (rok: 2021, ), Wydawca: Kraków, Instytut Katalizy i Fizykochemii Powierzchni im. Jerzego Habera PAN
    Data:
    konferencja 22 - 24 września
    Status:
    Published
  15. New approaches to generation of acid sites in mesoporous silicas
    Authors:
    M. Trejda, A. Nurvita, D. Kryszak, A. Jądrzak, M. Drobnik
    Conference:
    19th International Zeolite Conference; Zeolites make tommorrow better (rok: 2019, ), Wydawca: Organizatorzy Konferencji - Perth, Australia
    Data:
    konferencja 07-12 lipca 2020
    Status:
    Published
  16. The influence of Zr residues in short channel SBA-15 on state and activity of metallic modifiers (Ag, Au, Cu, Fe)
    Authors:
    Joanna Wisniewska, Kalina Grzelak, Shao-Peng Huang, Izabela Sobczak, Chia-Min Yang, Maria Ziolek
    Conference:
    14th EuropaCat - European Congress on Catalysis "Catalysis without Borders" (rok: 2019, ), Wydawca: Organizatorzy Konferencji - Kluby Katalizy: Niemcy, Holandia, Belgia
    Data:
    konferencja 18-23 sierpnia 2019
    Status:
    Published
  17. Anti-coke behaviour of silylated Nb/SBA-15 catalysts for glycerol dehydration
    Authors:
    K. Stawicka, M. Trejda, M. Ziolek
    Conference:
    8th Conference of the Federation of European Zeolite Associations (FEZA 2021) (rok: 2021, ), Wydawca: https://www.fezaconference.org/programme/virtual-programme-overview/
    Data:
    konferencja 5 - 9 lipca
    Status:
    Published
  18. Application of 3D and 2D zeolites as supports for gold catalysts addressed to selective base-free glucose oxidation to gluconic acid
    Authors:
    Adrian Walkowiak, Joanna Wolska, Anna Wojtaszek-Gurdak, Izabela Sobczak, Lukasz Wolski, Maria Ziolek
    Conference:
    9th World Congress on Oxidation Catalysis: Oxidation for a Sustainable Future and Clean Environment; Cardiff (rok: 2022, ), Wydawca: Organizing Commitee
    Data:
    konferencja 4-8 September 2022
    Status:
    Published
  19. Impact of sulphonic species on vanadium properties in SBA-15 material
    Authors:
    A. Nurwita, M. Trejda, P. Decyk, M. Ziolek
    Conference:
    8th Conference of the Federation of European Zeolite Associations (FEZA 2021) (rok: 2021, ), Wydawca: https://www.fezaconference.org/programme/virtual-programme-overview
    Data:
    konferencja 5 - 9 lipca
    Status:
    Published
  20. The effect of calcium dopant in Au-SBA-15 and Au-Nb/SBA-15 on the catalytic activity and selectivity in methanol oxidation
    Authors:
    J. Wisniewska, I. Sobczak, M. Ziolek
    Conference:
    8th Conference of the Federation of European Zeolite Associations (FEZA 2021) (rok: 2021, ), Wydawca: https://www.fezaconference.org/programme/virtual-programme-overview
    Data:
    konferencja 5 - 9 lipca
    Status:
    Published
  21. The way of gold location on pillars in MCM-36 zeolite
    Authors:
    Iveta Kaskow, Anna Wojtaszek-Gurdak, Izabela Sobczak
    Conference:
    14th EuropaCat - European Congress on Catalysis "Catalysis without Borders" (rok: 2019, ), Wydawca: Organizatorzy Konferencji - Kluby Katalizy: Niemcy, Holandia, Belgia
    Data:
    konferencja 18-23 sierpnia 2019
    Status:
    Published
  1. Silica Hosts for Acid and Basic Organosilanes: Preparation, Characterization, and Application in Catalysis
    Authors:
    Katarzyna Stawicka, Maria Ziolek
    Book:
    Chemistry of Silica and Zeolite-Based Materials; Synthesis, Characterization and Applications (rok: 2019, tom: Brak, strony: 27-56), Wydawca: Elsevier, ISBN 978-0-12-817813-3
    Status:
    Published

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