Projects funded by the NCN

Information on the principal investigator and host institution

Information of the project and the call

Keywords

Equipment

Delete all

Multifunctional catalysts for the production of carboxylic acids from the renewable sources

2018/29/B/ST5/00137

Keywords:

Acid-redox catalysts zeolites mesoporous materials charcteristic oxidation of glucose oxidehydration of glycerol tandem oxidehydration of ethanol

Descriptors:

  • ST5_3: Surface modification
  • ST5_6: Porous materials, ceramics, glasses
  • ST5_18:

Panel:

ST5 - Materials: materials synthesis, structure-properties relations, advanced and functional materials with designed properties, (macro)molecular architecture, material engineering

Host institution :

Uniwersytet im. Adama Mickiewicza w Poznaniu, Wydział Chemii

woj. wielkopolskie

Other projects carried out by the institution 

Principal investigator (from the host institution):

prof. Maria Ziółek 

Number of co-investigators in the project: 9

Call: OPUS 15 - announced on 2018-03-15

Amount awarded: 1 904 400 PLN

Project start date (Y-m-d): 2019-01-10

Project end date (Y-m-d): 2023-01-09

Project duration:: 48 months (the same as in the proposal)

Project status: Project settled

Project description

Download the project description in a pdf file

Note - project descriptions were prepared by the authors of the applications themselves and placed in the system in an unchanged form.

Equipment purchased [PL]

  1. Reaktor - kuweta IR.
  2. Chromatograf cieczowy HPLC (300 000 PLN)
  3. Kriostat.
  4. Auto-sampler do reaktora cieczowego Easy Max (140 000 PLN)
  5. Regulatory masowego przepływu.
  6. Rotor do wirówki.
  7. Spektrometr INVENIO-S Fourier Transform Infrared.
  8. Wirówka.

Information in the final report

  • Publication in academic press/journals (17)
  • Articles in post-conference publications (21)
  • Book publications / chapters in book publications (1)
  1. Calcium and nitrogen species loaded into SBA-15 – a promising catalyst tested in Knoevenagel condensation
    Authors:
    Dorota Kryszak, Katarzyna Stawicka, Maciej Trejda
    Academic press:
    Dalton Transactions (rok: 2020, tom: 49, strony: 9781), Wydawca: Royal Society of Chemistry
    Status:
    Published
    DOI:
    10.1039/d0dt01621g - link to the publication
  2. Gold-containing Beta zeolite in base-free glucose oxidation – The role of Au deposition procedure and zeolite dopants
    Authors:
    Joanna Wolska, Adrian Walkowiak, Izabela Sobczak, Lukasz Wolski, Maria Ziolek
    Academic press:
    Catalysis Today (rok: 2021, tom: 382, strony: 48-60), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.cattod.2021.05.020 - link to the publication
  3. The importance of residual water for the reactivity of MPTMS with silica on the example of SBA-15
    Authors:
    Katarzyna Stawicka, Maciej Gierada, Julia Gajewska, Frederik Tielens, Maria Ziolek
    Academic press:
    Applied Surface Science (rok: 2020, tom: 513, strony: 145802), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.apsusc.2020.145802 - link to the publication
  4. Enhancement of selectivity in methanol oxidation over copper containing SBA-15 by doping with boron species
    Authors:
    Zih-Yi Yang, Anna Wojtaszek-Gurdak, Chia-Min Yang, Maria Ziolek
    Academic press:
    Catalysis Today (rok: 2020, tom: 356, strony: 122-131), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.cattod.2019.06.035 - link to the publication
  5. Gold based on SBA-15 supports – Promising catalysts in base-free glucose oxidation
    Authors:
    Joanna Wisniewska, Izabela Sobczak, Maria Ziolek
    Academic press:
    Chemical Engineering Journal (rok: 2021, tom: 413, strony: 127548), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.cej.2020.127548 - link to the publication
  6. Niobium: The Focus on Catalytic Application in the Conversion of Biomass and Biomass Derivatives
    Authors:
    Luiz Oliveira, Márcio Pereira, Ana Pacheli Heitman, José Filho, Cinthia Oliveira and Maria Ziolek
    Academic press:
    Molecules (rok: 2023, tom: 28, strony: 1527), Wydawca: MDPI
    Status:
    Published
    DOI:
    10.3390/molecules28041527 - link to the publication
  7. The impact of Ce/Nb dopant ratio on basicity of MCF modified with calcium species
    Authors:
    Kalina Grzelak, Maria Ziolek, Maciej Trejda
    Academic press:
    Catalysis Communications (rok: 2020, tom: 142, strony: 106045), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.catcom.2020.106045 - link to the publication
  8. Insight into Active Centers and Anti-Coke Behavior of Niobium-Containing SBA-15 for Glycerol Dehydration
    Authors:
    Katarzyna Stawicka, Maciej Trejda, Maria Ziolek
    Academic press:
    Catalysts (rok: 2021, tom: 11, strony: 45309), Wydawca: MDPI
    Status:
    Published
    DOI:
    10.3390/catal11040488 - link to the publication
  9. Microwave-Assisted Base-Free Oxidation of Glucose with H2O2 on Gold- and Manganese-Containing SBA-15—Insight into Factors Affecting the Reaction Pathway
    Authors:
    Izabela Sobczak, Tsering Chödon Kowalska, Magdalena Nowicka and Maria Ziolek
    Academic press:
    International Journal of Molecular Sciences (rok: 2022, tom: 23, strony: 4639), Wydawca: MDPI
    Status:
    Published
    DOI:
    10.3390/ijms23094639 - link to the publication
  10. Modification of Gold Zeolitic Supports for Catalytic Oxidation of Glucose to Gluconic Acid
    Authors:
    Adrian Walkowiak, Joanna Wolska, Anna Wojtaszek-Gurdak, Izabela Sobczak, Lukasz Wolski, Maria Ziolek
    Academic press:
    Materials (rok: 2021, tom: 14, strony: 5250), Wydawca: MDPI
    Status:
    Published
    DOI:
    10.3390/ma14185250 - link to the publication
  11. The Impact of 3-(trihydroxysilyl)-1-propanesulfonic Acid Treatment on the State of Vanadium Incorporated on SBA-15 Matrix
    Authors:
    Ardian Nurvita, Piotr Decyk, Maria Ziolek, Maciej Trejda
    Academic press:
    Catalysts (rok: 2021, tom: 11, strony: 397), Wydawca: MDPI
    Status:
    Published
    DOI:
    10.3390/ - link to the publication
  12. The effect of support properties on n-octanol oxidation performed on gold – silver catalysts supported on MgO, ZnO and Nb2O5
    Authors:
    Iveta Kaskow, Izabela Sobczak, Maria Ziolek, Vicente Cortés Corberán
    Academic press:
    Molecular Catalysis (rok: 2020, tom: 482, strony: 110674), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.mcat.2019.110674 - link to the publication
  13. Towards efficient acidic catalysts via optimization of SO3H-organosilane immobilization on SBA-15 under increased pressure – potential application in gas and liquid phase reactions
    Authors:
    Maciej Trejda, Ada Kaszuba, Ardian Nurwita and Maria Ziolek
    Academic press:
    Materials (rok: 2021, tom: 14, strony: 7226), Wydawca: MDPI
    Status:
    Published
    DOI:
    10.3390/ma14237226 - link to the publication
  14. A platinum promoted Ag/SBA-15 catalyst effective in selective oxidation of methanol – design and surface characterization
    Authors:
    Joanna Wisniewska, Izabela Dziedzic, Maria Ziolek
    Academic press:
    RSC Advances (rok: 2020, tom: 10, strony: 14570), Wydawca: Royal Society of Chemistry
    Status:
    Published
    DOI:
    10.1039/d0ra01562h - link to the publication
  15. Activation of ethanol transformation on copper-containing SBA-15 and MnSBA-15 catalysts by the presence of oxygen in the reaction mixture
    Authors:
    Izabela Sobczak, Joanna Wisniewska, Piotr Decyk, Maciej Trejda and Maria Ziolek
    Academic press:
    International Journal of Molecular Sciences (rok: 2023, tom: 24, strony: 2252), Wydawca: MDPI
    Status:
    Published
    DOI:
    brak - link to the publication
  16. Development of a method for the synthesis of basic catalysts with high number of active species
    Authors:
    Katarzyna Stawicka
    Academic press:
    Catalysis Today (rok: 2020, tom: 354, strony: 51-60), Wydawca: Elsevier
    Status:
    Published
    DOI:
    10.1016/j.cattod.2019.09.013 - link to the publication
  17. The effect of the calcium dopant on the activity and selectivity of gold catalysts supported on SBA-15 and Nb-containing SBA-15 in methanol oxidation
    Authors:
    Joanna Wisniewska, Izabela Sobczak, Maria Ziolek
    Academic press:
    Catalysis Science & technology (rok: 2021, tom: 11, strony: 2242), Wydawca: Royal Society of Chemistry
    Status:
    Published
    DOI:
    10.1039/d0cy02135k - link to the publication
  1. Bimetallic AuAg catalysts supported on MgO, ZnO and Nb2O5 for noctanol oxidation: the effect of support and preactivation
    Authors:
    Iveta Kaskow, Izabela Sobczak, Maria Ziolek, Vicente Cortez Corberan
    Conference:
    14th EuropaCat - European Congress on Catalysis "Catalysis without Borders" (rok: 2019, ), Wydawca: Organizatorzy Konferencji - Kluby Katalizy: Niemcy, Holandia, Belgia
    Data:
    konferencja 18-23 sierpnia 2019
    Status:
    Published
  2. Insight into the factors affecting base-free glucose oxidation on gold-containing Beta zeolite – the role of Au deposition procedure and zeolite dopants
    Authors:
    J. Wolska, A. Walkowiak, I. Sobczak, L. Wolski, and M. Ziolek
    Conference:
    9th World Congress on Oxidation Catalysis: Oxidation for a Sustainable Future and Clean Environment; Cardiff (rok: 2022, ), Wydawca: Organizing Commitee
    Data:
    konferencja 4-8 September 2022
    Status:
    Published
  3. New approaches to generation of acid sites in mesoporous silicas
    Authors:
    M. Trejda, A. Nurvita, D. Kryszak, A. Jądrzak, M. Drobnik
    Conference:
    19th International Zeolite Conference; Zeolites make tommorrow better (rok: 2019, ), Wydawca: Organizatorzy Konferencji - Perth, Australia
    Data:
    konferencja 07-12 lipca 2020
    Status:
    Published
  4. Application of 3D and 2D zeolites as supports for gold catalysts addressed to selective base-free glucose oxidation to gluconic acid
    Authors:
    Adrian Walkowiak, Joanna Wolska, Anna Wojtaszek-Gurdak, Izabela Sobczak, Lukasz Wolski, Maria Ziolek
    Conference:
    9th World Congress on Oxidation Catalysis: Oxidation for a Sustainable Future and Clean Environment; Cardiff (rok: 2022, ), Wydawca: Organizing Commitee
    Data:
    konferencja 4-8 September 2022
    Status:
    Published
  5. Gold catalysts supported on 2D and 3D zeolites – characterization and application in base-free glucose oxidation
    Authors:
    Adrian Walkowiak, Joanna Wolska, Anna Wojtaszek-Gurdak, Izabela Sobczak, Lukasz Wolski, Maria Ziolek
    Conference:
    LIII Ogólnopolskie Kolokwium Katalityczne (rok: 2021, ), Wydawca: Powierzchni im. Jerzego Habera PAN
    Data:
    konferencja 22 - 24 września
    Status:
    Published
  6. The impact of Au deposition method on the catalytic performance of Beta zeolite-based gold catalysts in base-free glucose oxidation
    Authors:
    A. Walkowiak, J. Wolska, I. Sobczak, L. Wolski, M. Ziolek
    Conference:
    8th Conference of the Federation of European Zeolite Associations (FEZA 2021) (rok: 2021, ), Wydawca: https://www.fezaconference.org/programme/virtual-programme-overview/
    Data:
    konferencja 5 - 9 lipca
    Status:
    Published
  7. Wpływ metody wprowadzania Au na właściwości katalizatorów złotowych osadzonych na zeolicie Beta
    Authors:
    Adrian Walkowiak, Joanna Wolska, Izabela Sobczak, Łukasz Wolski, Maria Ziółek
    Conference:
    63. Zjazd naukowy Polskiego Towarzystwa Chemicznego (rok: 2021, ), Wydawca: PTChem
    Data:
    konferencja 13 - 16 września
    Status:
    Published
  8. Anti-coke behaviour of silylated Nb/SBA-15 catalysts for glycerol dehydration
    Authors:
    K. Stawicka, M. Trejda, M. Ziolek
    Conference:
    8th Conference of the Federation of European Zeolite Associations (FEZA 2021) (rok: 2021, ), Wydawca: https://www.fezaconference.org/programme/virtual-programme-overview/
    Data:
    konferencja 5 - 9 lipca
    Status:
    Published
  9. Ce and Nb as dopants in Ca/MCF system for enhancement of basicity
    Authors:
    K. Grzelak, M. Trejda, M. Ziolek
    Conference:
    8th Conference of the Federation of European Zeolite Associations (FEZA 2021) (rok: 2021, ), Wydawca: https://www.fezaconference.org/programme/virtual-programme-overview
    Data:
    konferencja 5 - 9 lipca
    Status:
    Published
  10. Influence of niobium and cerium dopants on optical and catalytic properties of gold catalysts supported on zeolite Beta
    Authors:
    Adrian Walkowiak, Joanna Wolska, Łukasz Wolski, Izabela Sobczak, Maria Ziółek
    Conference:
    LII Ogólnopolskie Kolokwium Katalityczne (rok: 2020, ), Wydawca: Kraków, Instytut Katalizy i Fizykochemii Powierzchni im. Jerzego Habera PAN
    Data:
    konferencja 25-27 XI
    Status:
    Published
  11. Microwave-assisted base-free oxidation of glucose with H2O2 on Au-MnSBA-15 and Cu-MnSBA-15 mesoporous sieves
    Authors:
    Izabela Sobczak, Tsering Kowalska, Magdalena Nowicka, Maria Ziolek
    Conference:
    Gold 2022 Conference; Quebeck City (rok: 2022, ), Wydawca: Organizing Commitee
    Data:
    konferencja 17-20 July 2022
    Status:
    Published
  12. The effect of water on the efficiency of MPTMS anchoring and its stability in mesoporous silica SBA-15
    Authors:
    Katarzyna Stawicka, Julia Gajewska, Maciej Gierada, Christina Siakati, Frederik Tielens, Maria Ziolek
    Conference:
    14th EuropaCat - European Congress on Catalysis "Catalysis without Borders" (rok: 2019, ), Wydawca: Organizatorzy Konferencji - Kluby Katalizy: Niemcy, Holandia, Belgia
    Data:
    konferencja 18-23 sierpnia 2019
    Status:
    Published
  13. Impact of sulphonic species on vanadium properties in SBA-15 material
    Authors:
    A. Nurwita, M. Trejda, P. Decyk, M. Ziolek
    Conference:
    8th Conference of the Federation of European Zeolite Associations (FEZA 2021) (rok: 2021, ), Wydawca: https://www.fezaconference.org/programme/virtual-programme-overview
    Data:
    konferencja 5 - 9 lipca
    Status:
    Published
  14. The effect of calcium dopant in Au/SBA-15 and Au/NbSBA-15 on the catalytic properties in oxidation of glucose and methanol
    Authors:
    J. Wisniewska, I. Sobczak, M. Ziolek
    Conference:
    15th Pannonian International Symposium on Catalysis (rok: 2022, ), Wydawca: toteMedia Lublin, Poland
    Data:
    konferencja 4-8 September 2022
    Status:
    Published
  15. The influence of Zr residues in short channel SBA-15 on state and activity of metallic modifiers (Ag, Au, Cu, Fe)
    Authors:
    Joanna Wisniewska, Kalina Grzelak, Shao-Peng Huang, Izabela Sobczak, Chia-Min Yang, Maria Ziolek
    Conference:
    14th EuropaCat - European Congress on Catalysis "Catalysis without Borders" (rok: 2019, ), Wydawca: Organizatorzy Konferencji - Kluby Katalizy: Niemcy, Holandia, Belgia
    Data:
    konferencja 18-23 sierpnia 2019
    Status:
    Published
  16. The role of water in SBA-15 on efficiency of MPTMS and APTMS anchoring
    Authors:
    Katarzyna Stawicka, Maciej Gierada, Julia Gajewska, Frederik Tielens, Maria Ziolek
    Conference:
    LII Ogólnopolskie Kolokwium Katalityczne (rok: 2020, ), Wydawca: Kraków, Instytut Katalizy i Fizykochemii Powierzchni im. Jerzego Habera PAN
    Data:
    konferencja 25-27 XI
    Status:
    Published
  17. Activity of MWW zeolites with different basic centers in Knoevenagel condensation
    Authors:
    Anna Wojtaszek-Gurdak, Vanesa Calvino-Casilda, Aneta Grzesinska, Rosa Martin-Aranda, Maria Ziolek
    Conference:
    14th EuropaCat - European Congress on Catalysis "Catalysis without Borders" (rok: 2019, ), Wydawca: Organizatorzy Konferencji - Kluby Katalizy: Niemcy, Holandia, Belgia
    Data:
    konferencja 18-23 sierpnia 2019
    Status:
    Published
  18. Base-free oxidation of glucose on Au/SBA-15 and Au/NbSBA-15 catalysts modified with calcium
    Authors:
    Joanna Wiśniewska, Angelika Wrublińska, Izabela Sobczak, Maria Ziółek
    Conference:
    LII Ogólnopolskie Kolokwium Katalityczne (rok: 2020, ), Wydawca: Kraków, Instytut Katalizy i Fizykochemii Powierzchni im. Jerzego Habera PAN
    Data:
    konferencja 25-27 XI
    Status:
    Published
  19. In search for the best bifunctional catalysts, based on MnSBA-15 and modified with Cu or Au, addressed to oxydehydration of glycerol
    Authors:
    Izabela Sobczak, Magdalena Nowicka, Maria Ziółek
    Conference:
    LIII Ogólnopolskie Kolokwium Katalityczne (rok: 2021, ), Wydawca: Kraków, Instytut Katalizy i Fizykochemii Powierzchni im. Jerzego Habera PAN
    Data:
    konferencja 22 - 24 września
    Status:
    Published
  20. The effect of calcium dopant in Au-SBA-15 and Au-Nb/SBA-15 on the catalytic activity and selectivity in methanol oxidation
    Authors:
    J. Wisniewska, I. Sobczak, M. Ziolek
    Conference:
    8th Conference of the Federation of European Zeolite Associations (FEZA 2021) (rok: 2021, ), Wydawca: https://www.fezaconference.org/programme/virtual-programme-overview
    Data:
    konferencja 5 - 9 lipca
    Status:
    Published
  21. The way of gold location on pillars in MCM-36 zeolite
    Authors:
    Iveta Kaskow, Anna Wojtaszek-Gurdak, Izabela Sobczak
    Conference:
    14th EuropaCat - European Congress on Catalysis "Catalysis without Borders" (rok: 2019, ), Wydawca: Organizatorzy Konferencji - Kluby Katalizy: Niemcy, Holandia, Belgia
    Data:
    konferencja 18-23 sierpnia 2019
    Status:
    Published
  1. Silica Hosts for Acid and Basic Organosilanes: Preparation, Characterization, and Application in Catalysis
    Authors:
    Katarzyna Stawicka, Maria Ziolek
    Book:
    Chemistry of Silica and Zeolite-Based Materials; Synthesis, Characterization and Applications (rok: 2019, tom: Brak, strony: 27-56), Wydawca: Elsevier, ISBN 978-0-12-817813-3
    Status:
    Published

O Narodowym Centrum Nauki

Finansowanie nauki

Współpraca zagraniczna

Centrum prasowe

Deklaracja dostępności
Przetwarzanie danych osobowych
Polityka cookies

Partnerzy